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• WVDP 1
DECOMMISSIONING PLAN WVDP PHASE 1 DECOMMISSIONING • consideration of The conceptual conceptual model for streambed streambed sediment was developed developed after consideration streams, plausible future land uses how residual radioactivity enters and moves though the streams, uses valleys, how humans might be exposed for the stream valleys, exposed to residual contamination contamination in the the streams or on the banks, banks, and plausible habits of a person who might spend time at the the conceptual model future . Such considerations led to selection of a conceptual streams in the future. appropriate determined to be an appropriate RESRAD. The RESRAD code was determined compatible with RESRAD. mathematical extensive use in evaluating evaluating potential doses from from mathematical model model based based on its extensive subsurface soil DCGL surface soil and its use in the surface surface soil DCGL and subsurface radioactivity in surface radioactivity models models for this project. As shown in Figure 55-10, 10, the contamination zone zone was assumed assumed to be on the stream conditions bank rather than in the stream itself. This model is consistent with typical conditions Frank's Creek downstream downstream of the Lagoon 3 outfall as shown by the the observed along Frank's radiological radiological control area in Figure 5-11 5- 11 represented represented by the roped-off area. area . ItIt is conservative conservative compared to having having the contamination contamination zone in the stream itself where water would act as as compared shielding shielding to reduce the direct direct radiation dose. dose . The photograph in Figure 5-11 was taken from just inside the project premises premises security fence looking upstream toward the southwest. The confluence confluence with Erdman Brook lies lies about 200 feet upstream upstream from where the people are standing and the Lagoon 3 outfall is about 500 feet from where the people people are standing. standing . • 5-11. Franks Creek Looking Upstream (2008 WVDP photo) Figure 5-11. conceptual model Key features features of this conceptual model include include the following: following : •* • Revision 2 Revision purposes was A person person spending spending time in the area of the streams for recreation purposes determined to be the appropriate appropriate member member of the critical group; the area is not suitable for farming, livestock grazing, farming , grazing, or residential residential use because because of the steep 5-35 5-35 WVDP PHASE PHASE 11 DECOMMISSIONING DECOMMISSIONING PLAN PLAN WVDP stream stream banks, banks , especially especially considering considering further further erosion erosion that that is likely likely to to occur occur as as discussed previously. previously. discussed *• In In this exposure exposure scenario scenario the the primary primary radiation radiation source source is is considered considered as as the the on the the stream stream bank. bank. The ability ability of sediment sediment to adsorb adsorb and and sediment deposited deposited on sediment dilute species species of of absorb radionuclides radionuclides would would be expected expected to to concentrate concentrate otherwise otherwise dilute absorb ions ions from the the water water (NRC (NRC 1977). 1977). The The water water in in the stream stream provides provides some shielding shielding and from radionuclides radionuclides in in sediments sediments on on the stream stream bottom, bottom, thus thus and separation separation from 11 ingestion pathways reducing reducing direct exposure exposure and incidental incidental ingestion pathways from those sources." sources. *• The located on The hypothetical hypothetical recreationist recreationist is assumed assumed to be be located on the contaminated contaminated stream bank for 104 104 hours per year, year, which which could involve spending spending two two hours hours per per day, two days days per week week for 26 26 weeks weeks aa year, year, reasonable reasonable assumptions assumptions considering considering day, the the local local climate. climate. *• located on the stream bank and is assumed to The contaminated assumed to contaminated zone zone of interest interest is located be three three meters meters (10 feet) wide and 333 meters meters (1093 (1093 feet) long, long , with a total area area of Y.. acre). 1000 square meters meters (approximately (approximately ¼ 1000 *• contaminated zone on the stream Having Having the the contaminated stream bank takes into account account aa situation situation where the the stream level might rise rise significantly significantly then fall again to a lower lower level. • The hypothetical recreationist is assumed hypothetical recreationist assumed to eat venison from deer whose flesh is contaminated radioactivity from contaminated with contaminated radioactivity contaminated stream banks, such such as from grazing on grass, grass, and and ingesting ingesting stream water. water. Consideration Consideration was given to both receptor location and stream bank bank geometry. Potential doses to a recreationist from impacted stream stream water will be less less significant significant than potential doses doses from the stream stream bank for the following reasons: reasons : "• It would be plausible for the hypothetical It hypothetical recreationist recreationist to spend more time on the the stream bank than immersed in stream water; water; •* The water would provide radiation radiation shielding for radioactivity in the streambed radiation;; sediment, which wou ld decrease potential dose from direct direct radiation would decrease potential sediment, •* While stream bank, bank, the external dose from surface water would be be While on the stream source; and compared with the dose from the stream negligible compared stream bank source; •* Neglecting erosion of the stream bank source leads to greater Neglecting greater doses than streambed,, where considering erosion of the source from the stream bank to the streambed significant shielding from surface surface water would reduce the dose. • • The stream bank geometry was assumed to be represented by a plane source of bank. Potential doses from alternative source contamination along the stream bank. contamination source reasons:: in this evaluation for the following reasons configurations were not included in the stream stream itself itself would in the Note that modeling of transport, transport, deposition, and concentrations concentrations of radionuclides in would involve consideration consideration decommissioning, and and involve Phase 11 of of the the decommissioning, on potential potential releases releases after Phase require assumptions assumptions on require time.. not considered at this time end-state, factors which are appropriately not of the Phase 2 end-state, 11 Revision 2 5-36 5-36 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • *• in doses similar Any dose variation variation due to a sloped stream bank would likely result in movement of the receptor and exposure exposure to an equivalent equivalent to level sources sources due to movement assumed to spend time moving the moving throughout the uniform dose dose (e.g. receptor receptor is assumed source area area and facing all directions for equal amounts of time); *• Although exposure exposure to a source source area wider than several meters is unlikely unlikely assumed to be externally externally exposed to considering the steep terrain, the receptor receptor is assumed conservatism; and a circular infinite plane plane source source for conservatism; •* the Because the mass balance balance model was used for the sediment sediment calculations, the parameter is not used in the calculations for water dependent dependent source width parameter pathways. All of the input parameters parameters for development development of the streambed sediment DCGLs appear appear in Appendix in Appendix C. Table 5-7 identifies selected key input parameters. Parameters for Streambed Development(') Streambed Sediment DCGL Development(1) Table 5-7. Key Input Parameters J ·Value Value Parameter (Units) Area of contaminated (M contaminated zone (m • 2 Basis Basis 1.0E+03 1.0E+03 Area on stream bank. Thickness contaminated zone (m) Thickness of contaminated (m) 1.0E+00 Conservative assumption. Fraction of year spent outdoors outdoors 1.2E-02 1.2E-02 104 hours (out of a total of 104 in 8760 hours per year) in area. Cover (m) Cover depth (m) 0 Contamination on surface. Contamination (m/y) rate (m/y) Contaminated zone erosion rate Contaminated 0 0 Conservative assumption.(2) Conservative assumption. (2) Well pump intake depth (m below water water table) 0 Only applicable applicable to farming. Well pumping rate (m /y) 0 Only applicable applicable to farming. Unsaturated zone thickness (m) Unsaturated 0 Contamination on stream surface. bank surface. )) 3 coefficient for Contaminated Contaminated zone distribution coefficient strontium (mL/g) strontium (mUg) 1.5E+01 1.5E+01 See Table C-2. Contaminated zone distribution coefficient coefficient for cesium (mUg) (mL/g) 4.8E+02 4.8E+02 See Table Table C-2. distribution coefficient Contaminated zone distribution coefficient for (mL/g) americium (mUg) 4.OE+03 4.0E+03 See Table Table C-2. NOTES: (1) normally NOTES: (1) See Appendix Appendix C for other input parameters. parameters. Metric units are used here because they are normally in RESRAD. used in (2) conservative because in no erosion erosion of the the source. source. (2) This assumption is conservative because it it results in In development development of the conceptual conceptual model, model, consideration consideration was given to protection protection of environmental and ecological resources, as well as human health. ItIt was determined that environmental • Revision 2 5-37 5-37 WVDP WVDP PHASE PHASE 1 1 DECOMMISSIONING DECOMMISSIONING PLAN PLAN changes to to the the model model or the radioactivity radioactivity cleanup cleanup criteria criteria will will be necessary necessary for for this this no changes 12 12 purpose. 5.2.4 5.2.4 Mathematical Mathematical Model Model As noted previously, As noted previously, RESRAD RESRAD (Yu, (Yu, et et al. al. 2001) 2001) is is used used as as the the mathematical mathematical model model for mrem/y per DCGL development. development. Version Version 6.4 6.4 was was used to calculate calculate the unit unit dose dose factors (in mrem/y of the the 18 18 radionuclides each of of the the three three exposure exposure scenarios. Unit Unit dose dose pCi/g) for each each of radionuclides in each pCi/g) factors factors were were then scaled scaled in Microsoft Microsoft Excel Excel to calculate calculate individual individual radionuclide radionuclide DCGLs DCGLs corresponding to 25 mrem mrem per year. corresponding • RESRAD was RESRAD was selected selected as the mathematical mathematical model for DCGL development development due to the the extensive use by DOE and and by NRC NRC licensees licensees in evaluating evaluating doses from residual extensive considers multiple radioactivity radioactivity at decommissioned decommissioned sites. The RESRAD RESRAD model model considers multiple exposure pathways for direct contact contact with with radioactivity, radioactivity, indirect indirect contact, and and food uptake, uptake, which are are pathways evaluated at the WVDP. the conditions being evaluated post-Phase 1 conceptual RESRAD RESRAD was was used with the post-Phase conceptual models described described previously to radionuclide source concentrations concentrations (i.e., generate generate doses for unit radionuclide (Le., dose per pCi/g of source). to The resulting resulting doses doses were were then scaled to the limiting acceptable acceptable dose (25 mrem mrem in aa year) to radionuclide specific DCGLs (see Appendix provide maximum provide the radionuclide Appendix C). For example, the maximum determined to be 1.7 estimated Cs-137 in surface surface soil was was determined estimated annual dose from 1 pCi/g of Cs-137 mrem, so the DCGL for 25 mrem per year is 25 divided divided by 1.7 1.7 or 14.8 14.8 pCi/g prior prior to accounting accounting for decay decay (see Table C-5). The calculated calculated DCGLs were then then input input into the the concentration to verify model model as the source source concentration verify that the dose dose limit of 25 mrem per year year was not exceeded. post-Phase 1 application of RESRAD to the post-Phase Among the general considerations considerations for the application decommissioning conceptual models were: decommissioning 12 •* the surface soil due to the groundwater pathways model for surface Use of the non-dispersion groundwater relatively large source area; •* balance model, instead of the less conservative conservative non-dispersion non-dispersion Use of the mass balance model, for the subsurface sediment models due to the relatively relatively subsurface and streambed sediment small source source areas; areas; and and • DOE Order 450.1, Environmental ProtectionProgram,requires that DOE Environmental Management 12 DOE Order 450.1, Environmental Protection Program, requires that DOE Environmental Management of the the air, air, management system to ensure protection of have an environmental facilities such as the WVDP have environmental management environmental; public public resources in in compliance with applicable environmental; water, land, and other natural and cultural resources includes Implementing guidance resource protection laws, regulations, and DOE requirements. Implementing health; and resource guidance includes and Terrestrial Terrestrial Doses to to Aquatic Aquatic and for Evaluating Radiation Doses A Graded GradedApproach Approach for DOE Standard Standard 1153-2002, 1153-2002, A DOE Evaluating Radiation ecological to evaluate potential adverse ecological concentration guides guides to biota concentration Biota. This guidance guidance includes the use of biota Biota. evaluate potential radionuclides. effects from exposure to radionuclides. in relation doses to aquatic and riparian animals and plants in potential annual doses evaluates potential The WVDP routinely evaluates radionuclide RESRAD-BIOTA computer code (DOE 2004) and radionuclide to the biota concentration guides using the RESRAD-BIOTA with the the These evaluations show compliance with inwater and streambed sediment. These concentrations measured in environmental monitoring and control program for Phase 11 of the URS 2009). The environmental guides (WVES and URS Order 450.1 450.1 during during the the with DOE DOE Order 1.8 would would ensure ensure compliance compliance with in Section 1.8 decommissioning described in decommissioning activities. Revision 2 5-38 5-38 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • •* The conservative conservative assumption the assumption of no erosion erosion for soil and sediment sources sources in in the development development of DCGLs, DCGLs, so there will be no source depletion from erosion. The RESRAD RESRAD model has limitations in this application application in that it was developed developed for soil exposures and therefore does does not specifically specifically address certain transport mechanisms mechanisms exposures associated associated with sediment, sediment, such as: •" Periodic saturation of the contaminated zone located located along a stream stream bank flood zone; zone; •* Erosion/scour of stream bank material material and subsequent subsequent downstream downstream deposition deposition to to the stream-bottom; stream-bottom; •* from Deposition of clean material onto the stream bank, bank, transported transported downstream downstream from unimpacted upstream locations; *• Variability concentrations due to fluctuation in flow rates during water concentrations during Variability in surface water storm events; " • Partitioning of contaminants between the surface water and stream-bottom stream-bottom sediment; and *• Variability moisture Variability of airborne airborne dust loads due to varying stream bank sediment moisture content. To address the simplifications model,, and still retain conservatism in simplifications of the conceptual model results,, the following assumptions model: the results assumptions were made for the sediment model: • *• The model will not allow the contaminated contaminated zone to be below the water table (as (as may periodically happen to the stream bank), therefore it was assumed that there assumed was no unsaturated unsaturated zone, and that the water table exists immediately immediately below the the source; source; •* conservatively selected selected to reflect soil on a The inhalation parameter parameter values were conservatively farm,, although stream bank sediment is likely to result in lower respirable farm respirable dust loadings; loadings; •" Contaminated groundwater discharge to the stream, where where itit is Contaminated groundwater is assumed to discharge impounded and contributes to fish bioaccumulation; impounded contributes bioaccumulation; •* Fish ingested from the stream are large enough to provide a significant number of meals each year, but are assumed assumed to only be exposed exposed to contaminated contaminated water and never swim to uncontaminated uncontaminated sections of the stream; stream; and •* In addition to assuming the fish are never In never in clean assumed assumed to eat only fish that are contaminated contaminated when, not support fish at all at the present time owning to typically present as shown in Figure Figure 5-11. 5-11 . water, the recreationist is in actuality, actuality, the stream will the small amount of water represents plausible conditions on the stream The conceptual conceptual model just described described represents banks and in the streambeds. It is considered in streambeds. It considered to be aa valid model for the long term in support of a Phase unrestricted release release,, that is, is, the site-wide removal Phase 2 strategy involving unrestricted alternative EIS. However, it would not necessarily serve as aa valid alternative in the Decommissioning EIS. • Revision Revision 2 5-39 5-39 DECOMMISSIONING PLAN WVDP PHASE 1 DECOMMISSIONING model ifif the Phase 2 sources were to be closed in place, place, as with the site-wide close-inalternative. place alternative. accounting for processes This limitation results from the model not accounting processes that could impact site-wide close-in-place close-in-place alternative. alternative. For example, example, the streams in the future under the site-wide unchecked erosion in impacts on the streams could could occur in the long term from unchecked in the the areas, and increased radioactive waste disposal areas, areas, surface surface water runoff from eroded areas, include seepage of contaminated groundwater streams. Such impacts could include groundwater into the streams. in increases increases in radionuclide concentrations in water in the streams as well as increases in contamination contamination in the sediment. • This limitation would be considered considered in any decision made by DOE to remediate remediate banks. Such remediation Phase 1 remediation during Phase sediment in the streams and on the stream banks. decommissioning decommissioning activities activities would require require a revision to this plan. plan . RESRAD input parameters parameters were were selected from the following sources, generally in the the order given based on availability: given •* Site-specific available, (e.g. groundwater groundwater and vadose zone zone Site-specific values values where available, parameters parameters such as the distribution coefficients coefficients listed in Table 3-20); •* Semi site-specific literature values, (e.g. from site-specific literature (e.g . physical physical values based on soil type from data and behavioral factors based on regional NUREG/CR-6697 (Yu, et al. 2000) NUREG/CR-6697 based Exposure Factors Handbook (EPA in the U.S. Environmental Environmental Protection Protection Agency's Exposure Factors Handbook 1997); •* Scenario-specific values using conservative Scenario-specific conservative industry defaults, (e.g., from the the Exposure Factors Factors Handbook, Exposure Handbook, the RESRAD RESRAD Data Data Collection Collection Handbook Handbook (Yu, et al. NUREG/CR-5512, Volume 1993), NUREG/CR-6697 NUREG/CR-6697 (Yu, et al. 2000), and NUREG/CR-5512, Volume 3 (Beyeler, (8eyeler, et al. 1999); •* parameters defined by aa The most likely values among default RESRAD parameters NUREG/CR-6697 (Yu, et distribution, when available, otherwise mean values from NUREG/CR-6697 distribution, al. 2000). 5.2.5 5.2.5 • Results Summary of Results Summary Table 5-8 provides provides the calculated individual individual radionuclide radionuclide DCGLs for surface surface soil, average subsurface subsurface soil, and streambed streambed sediment sediment which assure that the dose to the average the dose exceed 25 mrem per year when considering member of the critical group will not member radionuclide individually. Note that the surface soil DCGLs apply contribution contribution from each radionuclide subsurface soil contamination and only to areas of the project premises where where there is no subsurface that the subsurface subsurface soil DCGLs apply only to the bottoms and lower sides (extending (extending from from a depth of three feet and greater) of the large excavations in WMA 1 and WMA 2. 2. Table 5-8. DCGLs For 25 mrem pCi/g)(1) mrem Per Year (DCGLw (DCGLw Values in pCilg)(1) Nuclide Surface Surface Soil Subsurface Soil(3) Subsurface Streambed Sediment Streambed Sediment Am-241 4.3E+01 7.1 E+03 7.1E+03 1.6E+04 1.6E+04 C-14 2.OE+01 2.0E+01 3.7E+05 3.7E+05 3.4E+03 3.4E+03 Revision Revision 2 5-40 5-40 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • • 5-8. DCGLs For 25 mrem Per Year (DCGLw Table 5-8. (DCGLw Values in pCi/g)(1) Nuclide Surface Surface Soil Subsurface Subsurface Soil(3) Soil(3) Streambed Streambed Sediment Sediment Cm-243 4.1E+01 1.2E+03 1.2E+03 3.6E+03 3.6E+03 Cm-244 8.2E+01 8.2E+01 2.3E+04 4.8E+04 Cs-137(2) 2.4E+01 2.4E+01 4.4E+02 4.4E+02 1.3E+03 1.3E+03 1-129 1 -129 3.5E-01 3.5E-01 5.2E+01 3.7E+03 3.7E+03 Np-237 9.4E-02 9.4E-02 4.3E+00 4.3E+OO 5.2E+02 5.2E+02 Pu-238 5.0E+01 1.5E+04 1.5E+04 2.OE+04 2.0E+04 Pu-239 4.5E+01 1.3E+04 1.8E+04 Pu-240 4.5E+01 1.3E+04 1.3E+04 1.8E+04 Pu-241 1.4E+03 2.4E+05 5.1 E+05 5.1E+05 Sr-90(2) Sr-90(2) 6.3E+00 6.3E+OO 3.2E+03 9.5E+03 9.5E+03 Tc-99 Tc-99 2.4E+01 1.1 E+04 1.1E+04 2.2E+06 2.2E+06 U-232 5.8E+00 5.8E+OO 1.OE+02 1.0E+02 2.6E+02 2.6E+02 U-233 1.9E+01 1.9E+01 1.9E+02 5.7E+04 5.7E+04 U-234 2.OE+01 2.0E+01 2.OE+02 2.0E+02 6.0E+04 6.0E+04 U-235 1.9E+01 1.9E+01 2.1 2.1E+02 E+02 2.9E+03 2.9E+03 U-238 U-238 2.1E+01 2.1E+01 2.1E+02 1.2E+04 1.2E+04 NOTES: in NOTES : (1) Refer to Sections Sections 5.2.7 and 5.2.8 5.2.8 for discussions about how this th is set of DCGLs was considered considered in establishing establishing cleanup goals. goals. (2) Sr-90 and Cs-137 DCGLs reflect reflect 30 years years of decay and apply to the year 2041 and later. models. (3) The The lower deterministic DCGL of the resident farmer and residential gardener conceptual conceptual models. As noted previously, sum-of-fractions rule will be applied if characterization data previously, the sum-of-fractions if characterization indicate that a mixture of radionuclides radionuclides is present present in an area. area . indicate Conclusions About Results Results simulations are presented presented in Appendix C. C. For surface surface Detailed outputs of the RESRAD simulations soil, the results show that: soil , •" Am-241 doses are due primarily primarily to ingestion of plants, •" Cs-137 doses exposure, and doses are due primarily to external exposure, •" Sr-90 doses are due primarily to ingestion of plants. plants. The modeling to develop subsurface soil DCGLs indicated that: develop the subsurface *• Am-241 doses are due primarily to external exposure exposure and ingestion of impacted plants, plants, *• Cs-1 37 doses external exposure, exposure, Cs-137 doses are due primarily to external " • Sr-90 doses are due primarily to ingestion of impacted impacted plants and water, and *• subsurface soil are greater greater than those for the surface surface soil. DCGLs for subsurface The modeling to develop the streambed sediment DCGLs indicated that: that: • Revision 2 5-41 WVDP WVDP PHASE 1 DECOMMISSIONING DECOMMISSION ING PLAN •* incidental ingestion of sediment Am-241 doses are due primarily to incidental sed iment and to external exposure, exposure, •* external exposure, Cs-137 doses are due primarily to external exposure, as well as ingestion of venison, venison, •" Sr-90 doses are due primarily to ingestion ingestion of venison, and •" DCGLs for the sediment sediment source are orders of magnitude magnitude greater than those for surface soil. I • Conservatism Calculations Conservatism in Calculations A number of factors make the DCGLs calculated base-case model calculated using the initial base-case conservative. DCGLs, these factors include, include, for example, example, the relatively conservative. For the surface surface soil DCGLs, short local growing season season,, which makes it it likely that crop and forage yields will be less less than those assumed for the site. subsurface soil DCGLs, DCGLs, conservative For the subsurface conservative factors include: •* the hypothetical well (cistern) used in the As discussed discussed previously, the diameter of the hypothetical initial base-case base-case model at two meters (about 6.6 feet) is much larger the larger than the 13 diameter of a typical water well (eight inches) 13.. *• Use of the mass balance in that all balance model within RESRAD is conservative conservative in leachate reaches reaches the intake well. radionuclide inventory inventory in leachate *• Because of the relatively short local local growing season, season , itit is likely that crop/forage crop/forage site. yields will be less than those assumed for the site. DCGLs, conservative conservative factors include: For the streambed sediment DCGLs, • Based on limited available data, the typical thickness of the contaminated contaminated zone is likely smaller than the one meter (about 3.3 feet) value used used in the analysis. analysis. " • contamination will be found in the stream beds, beds, not data, most contamination Based on available data, on the banks. banks. " • It is unlikely that the incidental incidental ingestion rate (50 mg/d) for sediment will be It be contaminated area. exclusively from the contaminated " • It is assumed recreationist are impacted impacted by the It assumed that all fish ingested by the recreationist the source; however, however, itit is more likely that aa recreationist may streambed sediment source; ingest fish from other locations as well. *• Similarly, it is unlikely that the venison ingested will be impacted by streambed sediment sediment sources exclusively. exclusively. ItIt is more likely that exposure will be from both areas. impacted and non-impacted non-impacted areas. • With the larger diameter, much more contaminated soil and residual radioactivity would be brought to the With the larger diameter, much more contaminated soil and residual radioactivity would be brought to the surface where exposure through through various pathways. The The difference in volume volume would would vary vary with with surface where itit could could cause cause exposure various pathways. difference in the square of of the much contaminated soil would surface in inthe the radius; radius; 100 100 times times as as much contaminated soil would be be brought brought to to the the surface the the square conceptual model with with the the two meter diameter diameter well well than than with aa model that assumed assumed a 20 centimeter (eight conceptual model that centimeter (eight inch) diameter The larger assumed ensures pumping needs of the the residential inch) diameter well. well. The larger diameter diameter well well assumed ensures that that the the pumping needs of residential farm would be met, since a smaller diameter well could not do this on some parts of the project premises. premises. 13 13 Revision 2 5-42 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • • Assumptions regarding the availability availability of an adequate adequate fish population to allow allow long long term fish ingestion ingestion may also result in overestimation overestimation of doses doses related to the the sediment source, there are currently currently no fish in in the streams streams of sufficient quality or source, as there quantity for sustained human human consumption. DCGLs Applicability of Streambed Sediment Sediment DCGLs The conceptual model used for developing developing DCGLs for stream stream bed sediment in Erdman Brook and the portion of Franks Creek on the project premises streams premises assumed that these streams banks.. Th This parts. have steep banks is condition exists in most parts of the streams but not all parts. Consequently, itit is necessary necessary to define where the streambed Consequently, streambed sediment sediment DCGLs and cleanup cleanup goals apply. sediment DCGLs and cleanup Figure 5-12 shows the points where the streambed sediment cleanup apply. As indicated on the figure, figure , the surface soil DCGLs and cleanup goals apply goals apply. upstream upstream of these points and to the small tributaries tributaries to the streams. streams. • / Streambed sediment cleanup goals apply downstream of this point (surface soil cleanup goals apply upstream). Figure 5-12. Areas Where Streambed Sediment DCGLs and Cleanup Cleanup Goals Apply Figure 5-12. Apply • Revision 2 5-43 5-43 DECOMMISSIONING PLAN WVDP PHASE 1 DECOMMISSIONING 5.2.6 Analyses Discussion of Sensitivity Sensitivity Analyses Table performed for the surface soil DCGL Table 5-9 summarizes summarizes the sensitivity analyses analyses performed base-case C. base-case model, model , which are detailed in Appendix C. DCGLs(1) Surface Soil Parameter Sensitivity Analyses -- Surface Soil DCGLs(1) Table 5-9 Summary of Parameter Parameter Indoor/Outdoor Indoor/Outdoor Fraction Run 11 Change in Sensitivity Parameter Minimum Change Minimum DCGL DCGL Change Change -32% -32% -22% -22% Nuclide(s) U-232 Maximum DCGL DCGL Change Change Maximum Change 0% 0% Nuclide(s) 11-129 -129 2 21% 21% 0% 1-129 U-234 U-234 28% 28% 3 -50% -50% 9% U-232 81% 81% 4 200% 200% -28% -28% U-235 0% 5 -50% -50% -3% U-235 U-235 0% 0% 6 6 150% 150% 0% 12% 12% Irrigation/Pump Irrigation/Pump Rate 7 -57% -57% 8 8 70% 70% -1% -36% -36% Cs-1 37 Sr-90 U-232 U-232 U-232 U-232 1-129 1-129 Cs-I137 Cs-137 Sr-90 U-232 U-232 U-235 U-235 65% 65% 1% 1% 1-129 U-232 U-232 Soil/Water Distribution Coefficients (Kd) (I<d) 9 lower -71%% -71 U-234 U-234 0% Cs-137 Cs-1 37 10 10 higher higher -3% -3% U-232 U-232 867% 867% U-234 U-234 11 -55% -36% -36% 11-129 -1 29 0% 0% Cs-137 Sr-90 U-232 U-232 12 57% 57% 0% Cs-137 Sr-90 U-232 U-232 40% 40% 1-129 1-129 13 -23% -23% -29% -29% U-234 U-234 2% 2% U-232 U-232 14 15% 15% -2% -2% U-232 79% 79% 1 -1 29 1-129 15 15 -40% -40% -40% -40% 1-129 1-129 0.0% 0.0% Cs-1 37 Sr-90 Cs-137 Sr-90 U-232 16 16 100% 100% 0% Cs-1 37 Sr-90 Cs-137 U-232 99% 99% 1-129 1 -129 17 -30% -30% 0% Cs-1 37 Sr-90 U-232 U-232 30% 30% 1-129 1-129 18 18 21% 21% -12% -12% 1-129 0.0% 0.0% Cs-i137 Sr-90 Cs-137 U-232 19 19 -33% -33% -23% -23% 1-129 0.0% 0.0% Cs-i137 Sr-90 Cs-137 Sr-90 U-232 20 33% 33% 0% Cs-137 Sr-90 U-232 23.3% 23.3% 1-129 1 -1 29 21 -38% -38% 0% Cs-1 37 1-129 Sr-90 U-232 U-233 U-234 U-235 U-238 0.0% 0.0% Cs-137 1-129 1-129 Sr-90 U-232 U-232 U-233 U-234 U-234 U-235 U-238 U-238 Contamination Zone Thickness Unsaturated Zone Thickness Hydraulic Hydraulic Conductivity Runoff/ Evaporation Coefficient Depth of Well Intake Length Parallel Parallel to Aquifer Aquifer Flow Hydraulic Gradient Gamma Shielding Factor Revision 2 Revision 5-44 5-44 U-235 • 0% U-232 Sr-gO Sr-90 Cs-137 Cs-1 37 • • DECOMMISSIONING PLAN WVDP PHASE 11 DECOMMISSIONING • 1 DCGLs0 ' Soil DCGLs(1) Surface Soil Analyses -- Surface Parameter Sensitivity Analyses Table 5-9 Summary of Parameter Parameter Minimum DCGL Change Minimum DCGL Change Change 22 87% 87% -24% -24% 23 -60% -60% 24 Nuclide(s) Nuclide(s) Maximum DCGL Change Maximum DCGL Change Change Nuclide(s) U-232 0.0% 0.0% 1-129 0% 0% Cs-137 1-129 Cs-137 1-129 Sr-90 U-234 U-234 0.2% 0.2% U-232 U-232 -25% -25% 0% 0% Cs-137 Cs-1 37 1-129 1-1 29 Sr-90 U-233 U-233 U-234 U-234 0.1% 0.1% U-232 U-232 25 -70% 0% 0% Cs-137 1-129 Cs-1 37 1 -1 29 Sr-90 U-234 U-234 0.3% 0.3% U-232 26 67% 67% 0% U-232 0.0% 0.0% Cs-137 Cs-1 37 1-129 Sr90 U-235 U-238 Root Depth 27 27 -67% -67% 0% 0% Cs-137 1-129 Cs-137 Sr-90 U-232 U-232 U-233 U-234 U-235 U-238 0.0% 0.0% Cs-137 1-129 1-129 Cs-137 Sr-90 U-232 U-233 U-234 U-234 U-235 U-238 U-235 U-238 28 29 30 30 233% 233% Food Transfer Factors Factors lower higher higher 0% -38% -97% -97% 1-129 U-235 Sr-90 Sr-90 193.7% 193 .7% 875% 875% 42% -42% 31 31 NA -67% -67% U-234 0.0% 0.0% Indoor Dust Filtration Factor Filtration Dust Loading Factor Mass Balance Balance Model • Change in Change in Sensitivity Parameter Run I Sr-90 Sr-90 U-238 Cs-1 37 Sr-90 Cs-137 U-232 I U-232 contribute significantly significantly to to the here are are for radionuclides considered NOTES: (1 (1)) Results Results presented presented here NOTES: for radionuclides considered likely likely to to contribute the overall overall characterization data. surface surfa ce soil dose based based on available available characterization data. Results Discussion of Surface Soil Results model been evaluated The sensitivity analysis results for the surface soil source model drivers, i.e., that are the primary dose considering those radionuclides radionucl ides i.e ., those that are likely likely characterization data. The The available characterization to contribute significantly significantly to predicted predicted dose based on available uptake), 1-129 1-129 (due to water radionuclides radionuclides are Sr-90 (due to water independent independent plant uptake), uranium radionuclides radionuclides dependent pathways), dependent pathways), Cs-137 (external radiation dose), and most uranium (water dependent dependent pathways). pathways). the radionuclides, indicates The sensitivity analysis of the surface surface soil model, model , for these radionuclides, indicates the following: following : lower indoor indoor exposure exposure fraction decrease for U-232. •" A A lower fraction results results in the largest largest DCGL decrease U-232. Similarly, fraction results in the largest increase for U-232 Similarly, a higher indoor exposure fraction U-234. However, and no change change for 1-129 and U-234. However, itit is unlikely that the indoor fraction is climate.. The U-232 too low based on the local climate U-232 doses doses are mainly due to external exposure, which exposure, wh ich accounts accounts for the relative sensitivity sensitivity to this parameter. Decreasing the the source thickness increased increased the DCGL for all radionucl radionuclides •" Decreasing source thickness ides and increasing the source th thickness ickness resulted in the most significant significant DCGL decrease for parameter is due to increased/decreased U-235. The sensitivity to this U-235. th is parameter increased/decreased dose from independent). the water ingestion and plant pathways pathways (both water dependent dependent and independent). • Revision 2 Revision 5-45 5-45 WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN Decreasing the unsaturated U•" Decreasing unsaturated zone zone thickness thickness resulted in a decreased decreased DCGL for U235 and produced no change for Cs-137, 1-129, U-232.. Similarly, Similarly, increasing the I Cs-137, 1 - 129, and U-232 unsaturated zone thickness increased the U-235 DCGL and produced change unsaturated produced no change for Cs-137, 1-129, and U-232. Sensitivity to this parameter is mainly due to U-232. Cs- 137, 1-1 29, increased/decreased travel time of contaminants contaminants to the saturated zone, zone, resulting in increased/decreased water water dependent dependent doses occurring earlier/later earlier/later with respect to doses doses from water independent pathways. pathways. independent • Reducing the irrigation/well •" Reducing irrigation/well pump pump rate increased the DCGL for 1-129 most significantly. Similarly, significantly. Similarly, increasing the pump rate decreased decreased the DCGL for 1-129. 1-129. This This because reducing the pumping rate results in a lower dilution factor, is because factor, and radionuclide inventory available for increasing the pumping rate results in more radionuclide exposure. exposure. •" The most significant effects of varying the Kd Kd values were observed for U-234, U-234 , which Kd,d , to an increase ranged from aa decrease decrease of 71 percent percent when lowering the K increase of 867 867 Kd.. percent when increasing increaSing the ~ Decreasing the hydraulic conductivity 1-129 due •" Decreasing conductivity significantly reduced the DCGL for 1-129 due to reduced dilution pathways at the dilution and larger groundwater groundwater dose dose relative relative to other pathways the time of peak dose. increasing the hydraulic conductivity significantly dose. Similarly, increasing significantly increased the DCGL for 11-129. increased -129. runoff/evapotranspiration coefficients •" Variations Variations in the runoff/evapotranspiration coefficients had the greatest effect effect on U234 and 1-129, 1-129, and the least impact on U-232 U-232.. Radionuclides that are most sensitive to this parameter have doses mainly due to water water dependent dependent pathways. Decreasing the well decreased the DCGL for 1-129, 1-129, •* Decreasing we ll intake depth most significantly decreased while increasing th this parameter results in in significantly increased 1-129, increased the DCGL for 1-129, is parameter due to increased/decreased increased/decreased dilution in in the well water. Changes to contamination parallel •" Changes to the parameter parameter for length of contamination parallel to the aquifer flow flow DCGL, due to increased/decreased increased/decreased had the most significant significant effect on the 1-129 DCGL, dilution in the aquifer. • "• Changes Changes to the hydraulic gradient most significantly impacted 1-129, 1-129, due to the large significantly impacted large water dependent dependent pathway contributions. contributions. " Decreasing the the gamma shielding factor had no impact; however, increasing the • Decreasing the shielding shielding factor decreased the U-232 U-232 DCGL. "• Changes Changes to the indoor dust filtration factor had minimal impact DCGLs, due to impact on DCGLs, relatively larger pathways. larger contribution contribution to dose from other pathways. " Similarly, changes changes to the dust loading DCGLs, due to • Similarly, loading factor had minimal impact on DCGLs, relatively larger pathways. larger contribution to dose from other pathways. " Decreases in root depth did not significantly significantly impact DCGLs; however, however, increased increased impact the DCGLs; • Decreases root depths depths impacted Sr-90 most significantly due to relatively large plant pathway doses. doses. Revision 2 5-46 5-46 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSION ING PLAN • • Decreasing/increasing the plant transfer factors increased/decreased Decreasing/increasing factors significantly significantly increased/decreased the DCGL for Sr-90, Sr-90, as dose is mainly due to ingestion ingestion via plant uptake from soil. *• Use of the mass balance groundwater groundwater model significantly significantly decreases the DCGL for for Sr-90, Cs-137, Cs-137, or U-232 U-232.. Radionuclides most sensitive sensitive U-234 but had no effect effect on Sr-90, to this parameter dependent pathways. parameter have doses mainly due to water water dependent pathways. Table 5-10 summarizes summarizes the sensitivity analyses performed for the subsurface soil initial base-case model DCGLs, which are detailed in in Appendix C. Appendix C. base-case DCGLs, Table 5-10 Summary of Sensitivity Analyses - Subsurface Subsurface Soil DCGLs DCGLs Parameter • Change In in Sensitivity Parameter Parameter Indoor/Outdoor Indoor/Outdoor Fraction 1 2 2 -32% -32% Contamination Contamination Zone Thickness 3 4 4 Unsaturated Zone Unsaturated Thickness Thickness 5 6 Minimum DCGL Change Change Minimum DCGL Change Nuclide(s) Nuclide{s) -25% 0% 0% Cs-137 -67% -67% 233% 233% -65% -65% U-238 -4% -4% -1% -1% 6 -50% -50% 150% 150% 0% Irrigation/Pump Rate 7 8 -57% -57% 70% -39% -39% 0% C-3 r9 Cs-137 Sr-90 Cs 137 Sr 90 U-232 U-235 U-235 1-129 1 -1 29 Cs-137 Soil/Water SoillWater Distribution Distribution (Kd) Coefficients (Kd) Coefficients 99 lower -86% 10 10 higher higher -20% -20% Hydraulic Conductivity 11 12 12 -55% -55% 57% 57% 0% 0% 0% Runoff/ Runoff/ Evaporation Coefficient Coefficient 13 13 -23% -23% 14 14 Indoor Gamma Shielding Factor Indoor Dust Filtration Filtration Factor Inhalation Inhalation Dust Loading Root Depth Food Transfer Transfer Factors • Run Revision 2 8 21% 21 % 70% 0% 0% Maximum DCGL DCGL Change Change Maximum Change Change Nuclide(s) Nuclide{s) 0.3% 0.3% 35% 35% U-238 U-238 170% 170% 98% 98% Sr-90 U-232 U-232 1-129 1 -129 58% U-238 U-238 2218% 2218% U-234 1-129 1 -129 Cs-137 57% 57% 20% U-232 U-232 U-234 U-234 U-238 1-129 20% 1-129 U-238 116% 116% U-232 U-232 U-232 2168% 2168% U-234 U-234 no change 0% 0% no change change no 0% 0% no change no change change -44% -44% U-234 61% 61 % U-238 U-238 15% 15% -11 -11%% U-232 11 7% 117% U-234 U-234 15 15 16 16 -38% -38% 87% 87% 0% 0% -27% -27% U-238 19% 19% Cs-1 37 Cs-137 1% 1% U-232 U-232 U-238 U-238 17 -60% -60% 0% U-238 Cs-137 1-129 0% 0% U-235 U-235 18 18 -25% -25% 0% Cs-137 1-129 USr-90 U-233 UU-238 234 U-238 0% 0% U-235 U-235 19 19 -70% -70% 0% U-238 1% 1% 20 20 67% 67% 0% 0% U-235 U-235 0% 0% U-233 U-233 Cs-1 37 1-129 Sr9Cs-137 1-129 Sr90 90 21 21 -67% -67% -65% -65% Sr-90 1% 1% U-233 U-233 22 233% 233% lower higher 0% 0% -0.1% -0.1% -93% U-238 U-238 Sr-90 181% 181% 522% 522% 0% Sr-90 Sr-90 U-234 23 24 24 higher -93% 5-47 Sr-90 0% U-234 WVDP WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • Discussion Discussion of of Subsurface Subsurface Soil Soil Results Results The The sensitivity sensitivity analysis analysis results results for for the the subsurface subsurface soil source source initial base-case base-case model evaluated considering considering those those radionuclides radionuclides that that are are the primary primary dose drivers, drivers, i.e., i.e., were evaluated those those that are likely to contribute contribute significantly significantly to predicted predicted dose dose based based on on available available characterization data data (see Table 5-1). 5-1). The radionuclides radionuclides are are Sr-90 (due to water water characterization independent independent plant plant uptake), uptake), 1-129 1-129 (due to water water dependent dependent pathways), pathways), Cs-137 (external radiation radiation dose), dose), and and uranium uranium radionuclides radionuclides (water dependent dependent pathways). pathways). The sensitivity sensitivity analysis analysis of the subsurface subsurface soil model model for these radionuclides radionuclides indicates indicates the following: following : *• A lower lower indoor indoor exposure exposure fraction fraction results in aa DCGL decrease decrease for Cs-137 Cs-137 and and no no in a significant exposure results significant a significant significant change for U-238. U-238 . A higher indoor exposure results increased increased DCGL for U-232. U-232. However, However, it is unlikely that the indoor fraction is is too low low based on the local climate. climate. Doses for these isotopes isotopes are are mainly mainly due due to external based on exposure, which accounts accounts for the relative relative sensitivity to this this parameter. exposure, *• The source source thickness thickness parameter parameter sensitivity was most most significant for Sr-90, Sr-90, U-234, U-234, and U-238. increased/decreased dose dose U-238. The sensitivity sensitivity to this parameter parameter is due to increased/decreased pathways (both water from the water ingestion ingestion and plant pathways water dependent dependent and and independent). " • Decreasing or increasing increasing the the unsaturated unsaturated zone zone thickness thickness resulted in significant significant U-238.. changes for U-234 U-234 and U-238 • The 1-129 1-129 and U-238 DCGLs were were sensitive sensitive to changes changes in the irrigation/well irrigation/well pump pumping rate but the Cs-137 DCGL was not. This effect is because because reducing the pumping factor, and increasing increasing the pumping rate results in rate results in aa lower dilution factor, dependent pathways. more dilution for water water dependent pathways. *• U-232,, UUKd values were observed The most significant effects of varying the Kd observed for U-232 234, U-238. 234, and U-238. *• The hydraulic conductivity conductivity changes changes had no impact on DCGLs because because the mass used.. balance groundwater model was used *• The U-232 and U-234 DCGLs are sensitive to changes changes in the runoff/ Radionuclides that are most sensitive to this evapotranspiration evapotranspiration coefficient. Radionuclides this pathways. parameter have doses mainly due to water dependent dependent pathways. •* UChanges to the gamma shielding factor most significantly significantly impacted Cs-137 and U232, based on a relatively large external exposure dose. •* DCGLs, due to The indoor dust filtration factor variations had no impact on DCGLs, pathways. relatively large dose contributions from other pathways. •" Changes to the dust loading factor had a minimal impact on DCGLs, due to to relatively large dose contributions contributions from other pathways. •* Varying the root zone depth impacted the Sr-90 DCGL most significantly. Revision 2 5-48 I • • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • *• The plant transfer Sr-90,, as the dose is mainly due to transfer factor is most sensitive for Sr-90 ingestion via plant uptake uptake.. Table 5-11 5-11 Summary of Sediment DCGL DCGL Sensitivity Analysis Analysis In Change in Sensitivity Parameter Change Change 1 -50% 2% 2% 1-129 1 -129 97% 97% U-232 U-232 22 100% 100% -50% U-232 -3% -3% 1-129 1-129 3 -50% -50% 0% 0% U-235 29% Sr-90 44 200% -23% -23% U-233 0% Cs-137 Soil/Water Distribution Distribution Coefficients (Kd)) Coefficients (Kd 5 lower -76.5% -76.5% U-234 26% 26% U-232 6 6 higher higher -64.5% -64.5% U-233 U-233 52% 52% U-234 U-234 Runoff/Evaporation Runoff/Evaporation Coefficient 7 -23% -23% 15% 0% -3% Cs-137 8 4% 4% 0% U-232 U-232 Cs-1 37 Parameter Outdoor Fraction Fraction Source Thickness Mass Loading for Inhalation Root Depth • Food Transfer Factors Factors Run Minimum DCGL Change Minimum DCGL Change 8 15% -3% 9 9 -70% -70% 0% 0% 10 67% 67% 11 11 Nuclide(s) 1-129 1-129 Maximum DCGL Change Maximum DCGL Change Change Change Nuclide(s) Nuclide(s) 0% Cs-1 37 Cs-137 1-129 1-129 Sr-90 U-232 1% 1% U-233 U-233 -3% -3% U-234 0% Cs-137 1-129 Sr90 90 -67% -67% 0% 0% no change 0% no change change 12 233% 233% 0% U-232 U-235 50% 50% Sr-90 13 lower higher 1% 1% -98% -98% U-232 852% 852% Sr-90 Sr-90 Sr-90 -13% -13% U-232 U-232 14 14 higher Streambed Sediment Results Discussion of Streambed Results The streambed sediment model sensitivity simulations simulations have been evaluated considering considering those radionuclides radionuclides that are likely to significantly contribute contribute to the overall overall doses in this media, which are Sr-90 (venison ingestion) and and Cs-137 (external radiation dose). dose). The sensitivity model,, for these radionuclides, sensitivity analysis for the sediment sediment model radionuclides, indicates: • •" The DCGLs for Sr-90 and Cs-137 are inversely inversely related to changes changes in outdoor fraction, with Cs-137 being the most sensitive. sensitive. Radionuclides Radionuclides with primary doses from external parameter. external exposure exposure pathways are more sensitive to changes in this parameter. •" Decreasing the source thickness Cs-137. Decreasing thickness results in higher DCGLs for Sr-90 and Cs-137. While increasing the source radionuclides,, Sr-90 source thickness thickness has little effect effect on these radionuclides is most sensitive to this parameter. •* Varying the Kd Kd values had a minimal effect on the Cs-137 DCGL, DCGL, but decreasing decreasing the Kd decreased decreased the Sr-90 DCGL due to doses from water dependent pathways. Revision 2 Revision 5-49 DECOMMISSIONING PLAN WVDP PHASE 1 DECOMMISSIONING " • Varying Varying the runoff/evapotranspiration runoff/evapotranspiration coefficient had little effect on Cs-137 or Sr-90 to DCGLs. Radionuclides Radionuclides most sensitive to this parameter have doses mainly due to water dependent pathways. pathways. " • loading factor had minimal impact on DCGLs DCGLs.. Changes to the mass loading *• however, increasing the depth did not impact DCGLs; DCGLs; however, increasing the Decreasing the root zone depth depth increased increased the Sr-90 DCGL significantly. significantly. *• Decreasing both plant and fish transfer factors resulted in increased DCGLs for Srin decreased DCGLs for both Cs-137 90, and increasing these parameters parameters resulted in Cs-137 and Sr-90. • Changes to Base-Case Base-Case Models Based on Sensitivity Analysis Results Results Changes Development process Development of the conceptual conceptual model for surface surface soil DCGLs DCGLs was an iterative process assumptions for model parameters and took into account that used conservative conservative assumptions account the results of early model runs and the related input parameter parameter sensitivity analyses. analyses. The initial model runs produced inordinately low DCGLs for uranium radionuclides in radionuclides in calculated DCGLw example, was 1.0 pCi/g, surface soil. The calculated DCGL w for U-238, U-238 , for example, pCi/g , slightly above surface soil shown in Table 4-11 of this plan. plan . measured background concentrations concentrations in surface measured The next iteration involved changes to radionuclide radionuclide distribution coefficients. coefficients. Evaluation Evaluation of the basis for the original distribution distribution coefficients and sensitivity analysis results led to the the conclusion that some distribution coefficients coefficients used used were inappropriate. inappropriate. These distribution distribution coefficients were changed. The resulting distribution distribution coefficients coefficients are based either on sitespecific data for the sand and gravel layer or, where site-specific site-specific data are not available, values for sand from Sheppard and Thibault Thibault 1990, C-2. 1990, as shown in Table C-2. radionuclides, e.g., These model changes produced produced higher DCGLw DCGLw values for uranium radionuclides, e.g ., U-238. However, However, these values were still low compared 4.8 pCi/g for U-238. compared to uranium uranium DCGLs for unrestricted main unrestricted release developed developed at other sites. sites. Further evaluation evaluation showed showed that the main reason for the low uranium DCGLs was the conservative use of the RESRAD mass mass balance model. considering the results of the sensitivity analysis that evaluated evaluated use of model. After considering 14 14 the non-dispersion model model,, and RESRAD guidance ,, it was determined to be more more RESRAD Manual guidance appropriate to use the non-dispersion done. appropriate non-dispersion model in the surface surface soil analysis and this th is was done. • The probabilistic probabilistic uncertainty uncertainty analysis discussed in the next subsection SUbsection provided provided insight conservatism in model producing DCGLs that were model input parameters, parameters, producing were into the degree of conservatism analyses. generally lower than those from the deterministic deterministic analyses. 5.2.7 Probabilistic Uncertainty Analysis Analysis The probabilistic uncertainty uncertainty analysis has been performed performed for each of the three three conceptual models to supplement the deterministic sensitivity analyses just described. conceptual deterministic described . These probabilistic the probabilistic analyses generated generated results that quantify quantify the total uncertainty uncertainty in the 14 The RESRAD Manual (Yu, et al. 2001) notes Appendix E that:"The user has the option of selecting 14 The RESRAD Manual (Yu , et al. 2001) notes in in Appendix E that "The user has the option of selecting which [groundwater] model to use. the MB MB [mass [mass balance] is used for smaller smaller contaminated contaminated which [groundwater] use. Usually, Usually, the balance] model is areas (e.g., 1,000 m22 or less) and the ND [non-dispersion] model is used for larger areas." areas (e.g ., 1,000 m or less) and the ND [non-dispersion] model is used for larger areas ." Revision 2 5-50 5-50 • DECOMMISSIONING PLAN WVDP PHASE 1 DECOMMISSIONING • parameters, and also provide perspective DCGLs resulting from the variability of key input parameters, perspective regarding the relative relative importance of the contributions of different different input parameters to the the approach to DCGLs. This information supports a risk-informed approach uncertainty in the DCGLs. total uncertainty establishing cleanup goals for Phase 1 of the decommissioning. decommissioning . These analyses were performed performed using the probabilistic modules of RESRAD RESRAD version 6.4 , which utilize Latin hypercube hypercube sampling, sampling , a modified modified Monte Carlo method, method , allowing for 6.4, representative input parameter values from all segments segments of the input generation of representative the generation distributions. Input variables variables for the models were selected selected randomly from probability distributions. parameters treated distribution functions for each parameter of interest. The number of parameters distribution 102, subsurface follows:: surface soil 102, subsurface soil probabilistically for each conceptual conceptual model was as follows 67 , and streambed streambed sediment 63, with these figures including the biotransfer biotransfer factors and the the 67, (contaminated,, saturated saturated,, Kd values for the 18 18 radionuclides of interest for each zone (contaminated unsaturated) and media each each model. Appendix Appendix E provides details of the analyses. analyses . Table 5-1 5-11laa summarizes summarizes the results of the analyses. analyses. Probabilistic Uncertainty Table 5-11a. S-11a. Summary of Results of Probabilistic Uncertainty Analysesý') Analyses(1) Surface Soil DCGLs Subsurface Subsurface Soil DCGLs (pCi/g) (pCl'g) (pCi/g) Nuclide Nuclide Limiting Peak-ofDeterm(2) Peak-ofLimitin~ Determ(2) 3 3 the-Mean(3) the-Mean(3) ) Determ ) the.Mean( ) Determnn) the-Mean( • • DCGLs Streambed Sediment Sediment DCGLs (pCl'g) (pCi/g) Determ(5 ) Peak-of-the.Mean(3) Determ(5) Peak-of-the-Mean(3) Am-241 Am-241 4.3E+01 4.3E+01 2.9E+01 7.1EE+03 7.1 E+03 6.8E+03 1.6E+04 1.6E+04 1.OE+04 1.0E+04 C-14 2.0E+01 1.6E+01 1.6E+01 3.7E+05 3.7E+OS 7.2E+05 3.4E+03 3.4E+03 1.8E+03 1.8E+03 Cm-243 4.1E+01 4.1E+01 3.5E+01 3.SE+01 1.2E+03 1.IE+03 1.1E+03 3.6E+03 3.6E+03 3.1E+03 3.1E+03 Cm-244 8.2E+01 6.5E+01 6.SE+01 2.3E+04 2.2E+04 4.8E+04 3.8E+03 Cs-137(6) 2.4E+01 1.5E+01 1.SE+01 4.4E+02 3.OE+02 3.0E+02 1.3E+03 1.3E+03 1.0E+03 1.0E+03 1-129 3.5E-01 3.3E-01 5.2E+01 S.2E+01 6.7E+02 3.7E+03 3.7E+03 7.9E+02 Np-237 9.4E-02 2.6E-01 4.3E+00 4.3E+OO 9.3E+01 5.2E+02 5.2E+02 3.3E+02 3.3E+02 Pu-238 5.OE+01 5.0E+01 4.0E+01 1.5E+04 1.5E+04 1.4E+04 1.4E+04 2.OE+04 2.0E+04 1.2E+04 1.2E+04 Pu-239 4.5E+01 2.5E+01 2.SE+01 1.3E+04 1.3E+04 1.2E+04 1.2E+04 1.8E+04 1.2E+04 1.2E+04 Pu-240 4.5E+01 2.6E+01 1.3E+04 1.3E+04 1.2E+04 1.2E+04 1.8E+04 1.8E+04 1.2E+04 1.2E+04 Pu-241 1.4E+03 1.2E+03 1.2E+03 2.4E+05 2.4E+OS 2.5E+05 2.5E+05 5.1E+05 5.1E+05 3.4E+05 3.4E+OS Sr-90(6) Sr-90(6) 6.3E+00 6.3E+OO 4.1 E÷00 4.1E+OO 3.2E+03 3.4E+03 9.5E+03 9.5E+03 4.7E+03 Tc-99 2.4E+01 2.1E+01 1.1E+04 1.1E+04 1.4E+04 2.2E+06 2.2E+06 6.6E+05 6.6E+OS U-232 U-232 5.8E+00 5.8E+OO 1.5E+00 1.SE+OO 1.OE+02 1.0E+02 7.4E+01 7.4E+01 2.6E+02 2.2E+02 2.2E+02 U-233 1.9E+01 8.3E+00 8.3E+OO 1.9E+02 9.9E+03 9.9E+03 5.7E+04 2.2E+04 2.2E+04 U-234 2.0E+01 8.5E+00 8.SE+OO 2.0E+02 2.0E+02 1.3E+04 6.OE+04 6.0E+04 2.2E+04 2.2E+04 Revision 2 5-51 -------------------------~-. ~---- .. - - -_ .. - - --- WVDP WVDP PHASE PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN 5-11a. Summary Summary of of Results Results of of Probabilistic Probabilistic Uncertainty Uncertainty Analyses°• Analyses(l ) Table 5-11a. Surface Surface Soil Soil DCGLs DCGLs Subsurface Subsurface Soil Soil DCGLs (pCi/g) (pCi/g) Nuclide Nuclide (pCi/g) (pCi/g) Streambed Streambed Sediment Sediment DCGLs DCGLs (pCi/g) (pCilg) Peak-of- Limitin~ Limiting Determ ) Determ Peak-of-3 ) Peak-ofthe-Mean(3) the-Mean 5 Determ( Determ(5)) Peak-of-the-Mean(3) Peak-of-the-Mean(3) 2 Determ(2) ) Peak-ofDeterm( t3 the-Mean(3) the-Mean ) U-235 U-235 1.9E+01 1.9E+01 3.5E+OO 3.5E+00 2.1E+02 2.1E+02 9.3E+02 9.3E+02 2.9E+03 2.9E+03 2.3E+03 2.3E+03 U-238 U-238 2.1E+01 2.1E+01 9.8E+OO 9.8E+00 2.1E+02 2.1E+02 4.6E+03 4.6E+03 1.2E+04 1.2E+04 8.2E+03 8.2E+03 • NOTES : (1) Values Values shown shown in boldface boldface are are lower of of the the pair of of values va lues being being compared. compa red . NOTES: Revised deterministic deterministic DCGLs DCGLs based based on on parameter parameter changes changes described described in in Appendix Appendix C. C. (2) Revised (3) Probabilistic Probabilistic peak-of-the-mean peak-of-the-mean DCGLs DCGLs based based on analyses analyses described described in Appendix Append ix E. E. (4) These va lues are are the the limiting limiting DCGLs DCGLs for fo r subsurface soil soil from the residential residentia l gardener gardener alternate alternate scenario scenario These values 5.2.8, which describes in Section Section 5.2.8, describes discussed above. above. Subsurface soil DCGLs DCGLs are are discussed discussed further further in Subsurface soil analysis discussed the results an analysis that that takes into in to account continuing co ntinuing releases releases from from the bottoms bottoms of the the remediated results of an deep deep excavations. excavations. parameter (5) (5) These These are the revised DCGLs based based on para meter changes changes described described in Appendix Appendix C. C. (6) These values values take into account 30 years decay. decay. Table 5-1 5-11Iaa shows that: " • For surface surface soil, soil , the peak-of-the-mean peak-of-the-mean probabilistic probabilistic DCGLs are are lower lower than the the radionuclides except Np-237. revised deterministic DCGLs DCGLs for all radionuclides Np-237. *• soil, the limiting deterministic deterministic analysis analysis results results from the residential For subsurface subsurface soil, gardener alternative alternative scenario described described above are are more limiting than the peak-ofgardener the-mean radionuclides . (However, (However, the additional the-mean DCGLs for 10 of the 18 radionuclides. deterministic deterministic multi-source multi-source analysis analysis that includes continuing continuing releases releases from the the bottoms of the remediated excavations as discussed discussed in in Section Section 5.2.8 5.2.8 results results remediated deep excavations bottoms radionuclides of interest.) interest.) in even lower DCGLs for many of the radionuclides •* peak-of-the-mean DCGLs streambed sediment, sediment, the peak-of-the-mean For streambed DCGLs are more limiting than the the revised deterministic DCGLs. DCGLs. • th 95t" For most rad ionuclides, the 95 percentile probabilistic DCGLs are lower than the the most radionuclides, peak-of-the-mean DCGLs are peak-of-the-mean DCGLs as shown in Appendix E. peak-of-the-mean E. The peak-of-the-mean NRC considered considered to be appropriate to compare compare with the deterministic DCGLs because because NRC dose peak-of-the-mean dose modeling,, the peak-of-the-mean indicates that when using probabilistic dose dose modeling Rule compliance with its License distribution distribution should be used for demonstrating demonstrating compliance License Termination Rule 10 CFR 20, in 10 20, Subpart Subpart E (NRC 2006). 2006). After consideration of the results of the probabilistic probabilistic uncertainty analysis analysis and the analyses analyses of alternate alternate exposures exposures discussed previously, previously, DOE has determined determined that it is peak-of-the-mean DCGLs for surface soil appropriate appropriate to use the peak-of-the-mean soil and for streambed evaluations.. Subsurface soil sediment sediment and the lowest DCGLs of the various various subsurface soil evaluations DCGLs are addressed addressed in Section 5.2.8. 5.2.8 5.2.8 Multi-Source Analysis Analysis Subsurface Soil DCGL Multi-Source developing 5.2.1, the original base-case conceptual model used in developing As noted in Section 5.2.1, the subsurface soil DCGLs recognizes one source of contamination contamination - the Lavery till from Revision Revision 2 5-52 5-52 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • deep excavations surface during construction construction excavations that is brought to the surface the bottom of one of the deep groundwater potential impacts to groundwater hypothetical cistern. cistern . This model does not consider potential of the hypothetical backfilled excavation from continuing in the backfilled continuing release of remaining residual radioactivity radioactivity at the bottom of the deep excavations. excavations. limitation , analyses were performed performed that take into account account the impacts impacts To address this limitation, hypothetical residential gardener gardener of releases of this other residual radioactivity on both a hypothetical subsurface and a resident resident farmer with a modified model that accounts for a surface surface and a subsurface Figure 5-13 illustrates the modified modified conceptual conceptual model used in these radiation.. Figure source of radiation analyses. analyses. r zone Four surface contamination contamination zone geometry/dilution factor (DF) combinations geometry/dilution combinations 3 M3 plug of evaluated based on removal of a 3 m unweathered Lavery till to the surface: unweathered surface: 2 (1) 2000 M thick , with a soil DF of 100 100 m2 ,, 0.15 m thick, 2 (2) 2000 M thick, with aa soil DF of 1 m , 0.0015 m thick, 2 (3) thick, with a soil DF of 667 (3) 2000 M m2 ,, 1 m thick, 667 2 (4) 10,000 M ,, 1 m thick, 10,000 m thick, with aa soil DF of 3333 Ia A residential gardener average gardener is the average member of the critical group for the the 22 2000 M area scenarios. scenarios. A resident 2000 m the farmer is the average member2of the m2 the 10,000 critical group 10,000 m group for for the scenario. scenario. - lffýr -I - I -911 Backfill, unsaturated zone (2 m thick) Backfill , unsaturated in area where cistern Contamination Contamination on bottom of excavation in is installed is brought to surface surface and remaining subsurface contamination contributes to to groundwater source source contributes groundwater contamination • j Backfill, saturated Backfill, saturated zone zone Well (cistern) intake depth depth 5 m below water table] table 2 M2 ,, 1 m thick, thick, I Assumed 10,000 m Contamination diffuses into backfill early on located 10 m below surface Residual Radioactivity at Bottom of Excavation (Unweathered Lavery Till) Diffusion/dispersion spreads Diffusion/dispersion spreads contamination oetieShale contamination downward downward over time Hyw thetical cistern deep) 10 mn ca Bedrock. Figure 5-13. 5-13. Modified Conceptual Model for Subsurface Figure Subsurface Soil DCGL Development Development With this model model,, the subsurface soil DCGLs are based on exposure to residual radioactivity associated with the bottom of the deep unweathered Lavery deep excavation excavation in the unweathered installation till, surface during during insta llation of till , with (1) soil from this area assumed assumed to be relocated to the surface excavation bottom a cistern and (2) with the remaining contaminated contaminated Lavery till in the excavation • Revision 2 5-53 5-53 WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN serving as a continuing source source of contaminants contaminants to groundwater. groundwater. These sources and the the exposure pathways exposure pathways considered considered are described below. Excavation Bottom Contamination Excavation Bottom Treated Treated as Two Sources Sources of Contamination The excavation bottom is treated as two distinct sources: sources: (1) a plug of contaminated excavation bottom that is brought to the surface during installation of the the soil from the excavation garden , and (2) the remaining remaining cistern and spread over the entire surface of the hypothetical hypothetical garden, contaminated Lavery till at the excavation radioactivity moves contaminated excavation bottom from which residual radioactivity moves drawn into the well. Both the residential upward by diffusion and enters groundwater groundwater being drawn gardener scenario scenario and the resident farmer scenario were considered as indicated in Figure 5-13. 5-13. • The surface surface source source that results from the contribution contribution of contamination contamination in soil being removed from the bottom of the excavation excavation and brought to the surface and the contribution of contamination in irrigation irrigation water has the following characteristics: characteristics: *• It is assumed that the contaminated contaminated material It material is evenly spread across the entire hypothetical garden and mixed uniformly in the soil to varying depths depths (the surface hypothetical contamination zone), *• Exposure occurs from direct exposure and soil pathways pathways associated associated with surface, and contaminated soil brought to the ground surface, *• Exposure occurs from groundwater groundwater pathways pathways as contaminated contaminated water is drawn into the well and used as irrigation water resulting in plant contamination contamination and animal contamination where these plants are used as feed. As feed . a result, the resident is where used radioactivity from the plants being exposed to radioactivity being consumed consumed and, in the case of the the resident farmer scenario, scenario, from meat and milk produced from cattle that have been raised on the contaminated feedstock. feedstock. The subsurface subsurface source remaining at the bottom of the excavation is assumed assumed to have have characteristics: the following characteristics: " • The diffusive contamination from the excavation excavation bottom (the (the diffusive movement of contamination subsurface immediately after subsurface contamination zone) begins immediately after the excavation is contaminating the aquifer, backfilled and results in contaminating " • Contaminated groundwater groundwater entering the well is a source to soil in the surface surface garden,, and contamination zone because well water is used to irrigate the garden • Drinking water exposure occurs from contaminated contaminated well water being used as aa source of drinking water. source drinking • 5-1 lbb shows the exposure pathways Table 5-11 pathways evaluated. evaluated . Table 5-11 b. Exposure Pathways for Modified Subsurface Soil DCGL Model 5-11b. Exposure Pathways Residential Resident Residential Resident Exposure Pathways Farmer Gardener Farmer Gardener External gamma radiation radiation from contaminated soil Inhalation of airborne radioactivity radioactivity from re-suspended Inhalation re-suspended Revision 2 5-54 Yes Yes Yes Yes Yes Yes • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • Table 5-11b. Exposure Exposure Pathways for Modified Subsurface Subsurface Soil DCGL Model Residential Gardener Resident Resident Farmer Plant ingestion (produce impacted impacted by contaminated soil and groundwater groundwater contaminated contaminated by primary and secondary sources) Yes Yes Yes Meat ingestion (beef impacted impacted by contaminated soil and groundwater contaminated contaminated by primary primary and secondary sources) No Yes Yes Milk ingestion (impacted (impacted by contaminated contaminated soil and groundwater contaminated groundwater contaminated by primary and secondary sources) No Yes Yes Aquatic food ingestion Ingestion of drinking water (from groundwater groundwater contaminated by primary and secondary secondary sources) No No Yes Yes Yes Soil ingestion Yes Yes Yes Radon inhalation inhalation No No Exposure Pathways Exposure Pathways contaminated contaminated soil Details of the modeling including values of input parameters parameters such as distribution coefficients appear appear in the calculation calculation package (Price 2009). coefficients Mathematical Mathematical Models Models Calculation three-dimensional near combined dose utilized utilized information from the three-dimensional Calculation of the combined groundwater transport, transport, a model field STOMP finite difference difference model of the north north plateau for groundwater contamination from the subsurface subsurface that estimated estimated the drinking water dose associated with contamination source diffusing into the aquifer, aquifer, and RESRAD dose to source ratios associated associated with unit concentrations to determine pathways. The calculations were soil concentrations determine the total dose from all pathways. were implemented with a FORTRAN dependent implemented FORTRAN language computer program that estimates estimates time dependent impacts.1.155 human health impacts • concentrations over time The model performs mass balance balance calculations calcu lations and develops concentrations over time for three distinct distinct areas (1) the remaining subsurface source, source , (2) the backfilled saturated zone, and (3) the surface which has been contaminated the contaminated with material excavated from the subsurface source and radionuclides in irrigation water. subsurface radionuclides In order to identify controlling scenarios, the area of the contaminated contaminated zone In zone at the the surface and the degree garden were varied. varied. degree of mixing into the soil of the garden The STOMP model model was executed executed with parameter parameter values for the contaminated area and corresponded with assumptions used in the RESRAD well pumping rates that corresponded RESRAD model for the exposure scenarios under consideration consideration.. A contaminated area of 10,000 m2 and pumping pumping contaminated rate of 5720 m3/y were used to evaluate the resident farmer, and a contaminated contaminated area of 2 3 2,000 m m2 and well pumping rate of 1140 m 3/y were used to evaluate the residential gardener scenario. scenario. The residential residential gardener scenario scenario assumed assumed several source source 15These analyses were deterministic analyses. Consideration was given to performing probabilistic analyses These analyses were deterministic analyses . Consideration was given to performing probabil istic ana lyses instead. complexity of probabilistic analysis instead . However, However, the the complexity of the the multi-source multi-source model model made made aa probabilistic analysis impractical. impractical. 15 • Revision 2 Revision 5-55 5-55 WVDP PHASE 1 DECOMMISSION DECOMMISSIONING ING PLAN configurations within the contaminated contaminated area for the three m3 of contaminated contaminated Lavery till configurations excavated to the surface: assumed to be excavated " • Contamination is spread over the surface undiluted (1 .5 mm thick) of undiluted Contamination surface in a thin layer layer (1.5 till, till , *• Contamination is spread over Contamination over the surface surface and then tilled into the soil to a depth of 15 cm, and *• Contamination is spread Contamination spread over the surface surface and then tilled into the soil to a depth of 1 m. m. • determined to be most limiting for each radionuclide The source configuration configuration determined radionuclide was used as as the basis for the development of the subsurface DCGLs. subsurface DCGLs. Results Results Table 5-11 c shows the results of the analyses analyses compared compared to DGCLs developed developed using models.. other conceptual conceptual models Compar ison (pCi/g)(1) Table 5-11c. Subsurface Subsurface Soil DCGL Comparison (pCl/g)(11 Nuclide Nuclide Driller Recreat. Recreat. Hiker Hiker Lagoon 33 Natural Lagoon Natural Gas Gas Erosion Well Driller Erosion Well Driller Multi-Source Cistern Well Multi-Source Driller Basic Basic Deterministic Deterministic Delst Models(2) Models(2) Probabilistic Probabilistic Peak of thePeak of theMean Mean Mean Am-241 6.3E+03 1.7E+04 1.7E+04 2.7E+05 2.7E+OS 2.9E+05 2.9E+OS 1.4E+05 1.4E+OS 7.1E+03 6.8E+03 C-14 9.9E+02 2.3E+09 3.3E+08 6.4E+06 6.4E+06 4.9E+09 3.7E+05 3.7E+OS 7.2E+05 7.2E+OS Cm-243 3.6E+03 1.1E+04 1.1 E+04 5.OE+04 S.OE+04 1.8E+05 1.8E+OS 1.2E+05 1.2E+OS 1.2E+03 1.1E+03 1.1E+03 Cm-244 3.4E+04 3.3E+04 3.3E+04 1.0E+09 3.9E+05 3.9E+OS 2.6E+05 2.6E+OS 2.3E+04 2.2E+04 2.2E+04 Cs-137(3) Cs-1 37(3) 2.8E+03 6.7E+03 6.7E+03 9.8E+05 9.8E+OS 7.4E+05 7.4E+OS 9.2E+04 4.4E+02 3.OE+02 3.0E+02 1-129 7.5E+00 7.SE+OO 8.OE+05 8.0E+OS 1.9E+06 3.5E+05 3.SE+OS 9.2E+06 5.2E+01 S.2E+01 6.7E+02 Np-237 1.OE+00 1.0E+OO 6.6E+03 6.6E+03 2.7E+04 5.9E+05 S.9E+OS 6.6E+04 4.3E+00 4.3E+OO 9.3E+01 Pu-238 1.3E+04 1.3E+04 2.OE+04 2.0E+04 1.5E+06 1.SE+06 2.7E+05 2.7E+OS 1.6E+05 1.6E+OS 1.5E+04 1.SE+04 1.4E+04 1.4E+04 Pu-239 3.1E+03 1.9E+04 2.8E+05 2.8E+OS 2.4E+05 2.4E+OS 1.5E+05 1.SE+OS 1.3E+04 1.2E+04 1.2E+04 Pu-240 Pu-240 3.4E+03 1.9E+04 2.8E+05 2.8E+OS 2.4E+05 2.4E+OS 1.5E+05 1.SE+OS 1.3E+04 1.3E+04 1.2E+04 1.2E+04 Pu-241 5.5E+05 S.SE+OS 5.5E+05 S.SE+OS 1.7E+07 1.2E+07 4.5E+06 4.SE+06 2.4E+05 2.4E+OS 2.5E+05 2.SE+OS Sr-90(3)3 Sr-90( ) 2.8E+02 8.7E+05 8.7E+OS 1.6E+08 9.2E+06 1.1E+07 1.1 E+07 3.2E+03 3.4E+03 Tc-99 5.9E+02 S.9E+02 7.9E+07 2.2E+08 2.2E+08 4.7E+07 9.4E+08 1.1E+04 1.4E+04 1.4E+04 U-232 8.8E+01 1.6E+03 2.8E+04 4.5E+05 4.SE+OS 1.6E+04 1.0E+02 7.4E+01 U-233 2.7E+02 6.2E+04 1.3E+06 2.9E+06 4.9E+05 4.9E+OS 1.9E+02 1.9E+02 9.9E+03 U-234 2.8E+02 6.4E+04 1.4E+06 3.1E+06 3.1E+06 5.OE+05 S .OE+OS 2.OE+02 2.0E+02 1.3E+04 1.3E+04 U-235 U-23S 2.9E+02 1.2E+04 4.2E+04 3.2E+06 1.4E+05 1.4E+OS 2.1E+02 9.3E+02 U-238 3.OE+02 3.0E+02 3.7E+04 1.9E+05 1.9E+OS 3.3E+06 3.6E+05 3.6E+OS 2.1E+02 4.6E+03 • NOTES: NOTES: (1) The lowest DCGLs are shown in boldface. boldface. deterministic resident farmer and residential gardener gardener DCGLs. DCGLs. (2) The lower value of the deterministic (3) These values take into account 30 years decay. Revision 2 5-56 5-56 • WVDP WVDP PHASE PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN PLAN • In In nine nine cases, cases , the the DCGLs DCGLs developed developed using using other other conceptual conceptual models are are lower lower than the the DCGLs DCGLs developed developed by by the multi-source multi-source model that accounts accounts for continuing continuing releases releases from from the the the deep deep excavations: excavations: bottom of the *• The probabilistic DCGLs, DCGLs, which which did did not take take into into account account The peak-of-the-mean peak-of-the-mean probabilistic are lower for Cmexcavations, excavations, are lower Cmcontinuing releases from the bottom bottom of the deep continuing releases 243, Cm-244, Cm-244, Cs-137, Cs-137, and and U-232; U-232 ; and and 243, *• The The limiting limiting deterministic deterministic DCGL from the deterministic deterministic resident farmer and and residential gardener gardener conceptual conceptual models, models, which which did did not take take into account account continuing continuing U-234, releases releases from the bottom of the excavations, excavations, was lower for Pu-241, Pu-241 , U-233, U-233 , U-234, U-235, and and U-238. U-238. U-235, This situation can be be attributed attributed to conceptual conceptual model model differences differences such as as different different contamination contamination zone geometry. geometry. Conclusions 5.2.9 5.2.9 Overall Overall Conclusions iterative process. Development of DCGLs proved Development proved to be an iterative process. be DCGLs, the initial-base For surface surface soil soil DCGLs, initial-base case conceptual conceptual model was determined determined to be conservative than more conservative than an alternate alternate conceptual conceptual model involving erosion erosion and the resulting probabilistic peak-of-the-mean DCGLs potential doses doses to an offsite offsite receptor. receptor. However, However, the probabilistic peak-of-the-mean DCGLs base-case deterministic deterministic DCGLs were were lower than the base-case DCGLs for all all radionuclides radionuclides except Np-237. Np-237. The peak-of-the-mean DCGLs The peak-of-the-mean DCGLs were therefore therefore selected as the basis for the surface soil cleanup cleanup goals to be conservative. conservative . • For subsurface subsurface soil DCGLs, DCGLs, analysis analysis of the residential residentia l gardener and the multisource multisource alternate conceptual conceptual models models showed that the initial base-case base-case resident resident farmer model was was into provided additional insight into not conservative. conservative. The The probabilistic probabilistic uncertainty uncertainty analysis provided deep excavations. In at the bottom of the doses from residual radioactivity potential future excavations. In future bottom the interest of conservatism, conservatism, the lowest DCGLs DCGLs produced by the various models were were selected as the basis for the subsurface subsurface soil cleanup cleanup goals. the base-case model produced essentially For streambed sediment DCGLs, the refined base-case essentially the peak-of-the-mean base-case model. However, the probabilistic peak-of-the-mean same DCGLs as the initial base-case DCGLs were lower and were therefore therefore selected as the basis for the cleanup goals. 5.3 Assessment Limited Site-Wide Dose Assessment Limited This section describes the limited integrated dose assessment assessment performed performed to ensure activities will not limit options for Phase 2 of the in Phase 1 remediation that criteria used in remediation activities decommissioning.. decommissioning 5.3.1 Assessment Basis for this Assessment the appropriate,, considering the Section 5.1.3 explains why such a dose assessment assessment is appropriate the 5-4. Section 5.1.3 also explains that the Figure 5-4. Phase 1 and Phase 2 sources illustrated in Figure appropriate dose assessment involves a hypothetical individual engaged in farming at appropriate remediated project premises who also spends some time in the future on one part of the remediated spends time fishing and hiking at Erdman Brook and Franks Creek. • Revision 2 5-57 5-57 I WVDP PHASE 11 DECOMMISSIONING WVDP DECOMMISSIONING PLAN This scenario would involve an individual being exposed to two different remediated different critical groups. groups. As described source areas and being a member of the two different described in Section 5.2, exposure group for the resident resident farmer scenario scenario used for development of 5.2, the exposure DCGLs for surface and subsurface exposure group for subsurface soil is significantly different different from the exposure the development development of the streambed streambed sediment sediment DCGLs, which involves a hypothetical individual spending hunting individual spending a relatively small fraction of his or her time hiking, hiking, fishing, fishing , and hunting in the areas of Erdman Brook and Franks Creek. Creek. • In both of these cases, hypothetical individual (the average average cases, it was assumed that the hypothetical member of the critical group) would be exposed only to the residual radioactivity of interest. That is, the resident farmer would not be exposed to residual radioactivity in the areas of the streams streams and the recreationist would not be exposed exposed to residual radioactivity in surface surface soil or subsurface subsurface soil. 5.3.2 Assessment Approach Approach Assessment The approach approach used involves involves partitioning doses between between two critical groups and two (1) the resident in an area of the project premises where areas of interest: (1) resident farmer who lives in surface soil or subsurface subsurface soil has been remediated to the respective DCGLs and (2) (2) the the person who spends time in the areas of the streams hiking, fishing, and hunting (the This in recreationist). Th is approach approach is analogous analogous to addressing addressing multiple radionuclides radionuclides in contaminated media of interest (NRC contaminated interest using the sum-of-fractions sum-of-fractions approach or unity rule (NRC 2006). Consideration different areas led assigning Consideration of potential potential risks related to the different assigning 90 percent of the total dose limit of 25 mrem per year to the resident farmer farmer activities activities and 10 10 percent percent to activities.. This arrangement arrangement involves 22.5 the recreational recreational activities involves assigning an acceptable acceptable dose of 22 .5 mrem per year to resident resident farmer activities activities and 2.5 mrem per year to recreation recreation in the area area 16 of the streams, values values which total 25 mrem per year. year.1 6 The assessment assessment was then performed using the base case analysis results for the resident farmer and the recreationist performed at Erdman Brook and Franks Creek. • Two separate assessments were performed performed with the resident farmer located located in: in : (1) the the area of the remediated remediated WMA subsurface soil excavation, WMA 1 subsurface excavation, and (2) the resident resident farmer located remediated.. Details located in an area where surface surface soil was assumed to have been remediated Details appear in Appendix C. C. 5.3.3 Results of the Assessments Assessments subsurface soil case and Table 5-12 provides the assessment assessment results for the WMA 1 subsurface Table Table 5-13 provides the results for the surface surface soil case. The streambed streambed sediment DCGLw DCGLw values are the same in both cases because the apportioned apportioned dose limit of 2.5 2.5 mrem per year is the same. 16 This 0.9010.10 0.90/0.10 split is based judgment related related to relative risk. Consideration was 16 This split is based on on judgment to relative risk. Consideration was given given to to using a split split based on on the the relative relative time the the hypothetical hypothetical farmer would would spend spend in in the the area of the the farm compared to to the area area of the streams. However, because because the the assumed time time in in the the area of of the streams is is relatively small at 104 of streams . However, relatively small 104 hours per year, such as spilt could result in in an allowable allowable annual dose of 24.7 mrem for resident farmer activities and 0.3 mrem for recreation at the streams. streams . This split would have a minimal impact on the soil DCGLs while driving the streambed sediment DCGLs to unrealistically unrealistically low levels. Revision Revision 2 5-58 5-58 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • • Table 5-12. Site-Wide Dose Assessment 1I Results (DCGLs in pCi/g) 5-12. Limited Site-Wide Nuclide Nuclide Subsurface DCGLw Subsurface Soil DCGL w Values Base Case(1 ) Assessment(2) Base Case(1) Assessment(2) Streambed DCGLw Streambed Sediment DCGL Values w Values 1 Base Case( Assessment(2) Base Case(1)) Assessment(2) Am-2411 Am-24 6.3E+03 5.7E+03 C-1 4 C-14 9.9E+02 9.9E+02 8.9E+02 8.9E+02 1.8E+03 1.8E+03 1.8E+02 1.8E+02 Cm-243 Cm-243 1.1E+03 9.9E+02 9.9E+02 3.1E+03 3.1E+03 3.1E+02 3.1E+02 Cm-244 2.2E+04 2.OE+04 2.0E+04 3.8E+04 3.8E+04 3.8E+03 3.8E+03 3 Cs-137(3) Cs-137( ) 3.0E+02 2.7E+02 1.0E+03 1.OE+03 1.0E+02 1.OE+02 1-129 1-129 Np-237 Np-237 7.5E+00 7.5E+OO 1.OE+00 1.0E+OO 6.8E+00 6.8E+OO 9.0E-01 7.9E+02 7.9E+02 3.2E+02 3.2E+02 7.9E+01 3.2E+01 Pu-238 Pu-239 1.3E+04 3.1E+03 1.2E+04 2.8E+03 2.8E+03 1.2E+04 1.2E+04 1.2E+03 1.2E+03 1.2E+04 1.2E+04 1.2E+03 1.2E+03 Pu-240 Pu-240 Pu-241 Pu-241 3.4E+03 2.4E+05 3.1E+03 3.1 E+03 2.2E+05 2.2E+05 1.2E+04 1.2E+04 1.2E+03 1.2E+03 3.4E+05 3.4E+05 3.4E+04 3.4E+04 Sr-90(3) Sr-90(3) 2.8E+02 2.5E+02 2.5E+02 4.7E+03 4.7E+02 Tc-99 5.9E+02 5.3E+02 5.3E+02 6.6E+05 6.6E+05 6.6E+04 6.6E+04 U-232 U-232 U-233 7.4E+01 1.9E+02 6.7E+01 6.7E+01 1.7E+02 1.7E+02 2.2E+02 2.2E+02 2.2E+04 2.2E+04 2.2E+01 2.2E+03 2.2E+03 U-234 2.0E+02 1.8E+02 1.8E+02 2.2E+04 2.2E+04 2.2E+03 2.2E+03 U-235 2.1E+02 2.1 E+02 2.1 2.1E+02 1.9E+02 1.9E+02 2.3E+03 2.3E+03 8.2E+03 8.2E+03 2.3E+02 2.3E+02 8.2E+02 U-238 1.0E+04 1.OE+04 1.0E+03 1.OE+03 NOTES:: (1) (1) The base-case values for subsurface soil are 5-1 lcc and the base-case base-case NOTES are the lowest lowest values val ues from from Table 5-11 5-1111 a. values for streambed streambed sediment are are the lowest values from Table Table 5a. (2) The results for the analysis combined in th this in the the analysis of the com bined base-case in is table (the lowest lowest DCGLs in (2) analyses for subsurface recreationist in in the area of the th e streams. stream s. various analyses subsurface soil) and the recreationist (3) These DCGLs DCGLs apply in in the th e year 2041 and later. 5-13, the dose partitioning DCGLw As can be seen from Table 5-13, partitioning approach reduced the DCGL w values for surface soil by 10 percent and reduced DCGLww values for streambed reduced the DCGL magnitude. sediment by an order of magnitude. Table 5-13. Limited Site-Wide Site-Wide Dose Dose Assessment Assessment 2 Results (DCGLs in pCi/g) Nuclide Nuclide • Surface Soil DCGLw DCGLw Values 1 Base Case( Case(1) Assessment(2 Assessmentf 2 ) Values Streambed Sediment DCGLw DCGLw Values 1 Base Case(1) Assessment(2) Base Case( ) Am-241 2.9E+01 2.6E+01 2.6E+01 1.OE+04 1.0E+04 1.0E+03 1.0E+03 C-14 14 C- 1.6E+01 1.6E+01 1.5E+01 1.5E+01 1.8E+03 1.8E+03 1.8E+02 Cm-243 3.5E+01 3.5E+01 3.1E+01 3.1 E+01 3.1E+03 3.1E+02 Cm-244 Cs-137(3) Cs-137(3) 6.5E+01 6.5E+01 5.8E+01 3.8E+04 3.8E+03 1.5E+011 1.5E+0 1.4E+01 1.4E+01 1.OE+03 1.0E+03 1.0E+02 1.0E+02 1-129 1 -129 3.3E-01 2.9E-01 7.9E+02 7.9E+01 Np-237 2.6E-01 2.3E-01 3.2E+02 3.2E+01 Pu-238 4.0E+01 3.6E+01 1.2E+04 1.2E+04 1.2E+03 1.2E+03 Revision Revision 2 5-59 5-59 WVDP PHASE PHASE 11 DECOMMISSIONING DECOMMISSIONING PLAN P LAN WVDP Table 5-13. 5-13. Limited limited Site-Wide Site-Wide Dose Dose Assessment Assessment 2 Results Results (DCGLs (DCGLs in pCi/g) pCi/g) Table Nuclide Nuclide Surface Surface Soil Soil DCGLw DCGLw Values Values 1 Assessment(2) Base Case( Case(1) Base Streambed Streambed Sediment Sediment DCGLw DCGLw Values Values 1 Assessment(2) ) Case( Base Base Case(1) Assessment(2) Pu-239 Pu-239 2.5E+01 2.5E+01 2.3E+01 2.3E+01 1.2E+04 1.2E+04 1.2E+03 1.2E+03 Pu-240 Pu-240 2.6E+01 2.6E+01 2.4E+01 2.4E+01 1.2E+04 1.2E+04 1.2E+03 1.2E+03 Pu-241 Pu-241 1.2E+03 1.2E+03 1.OE+03 1.0E+03 3.4E+05 3.4E+05 3.4E+04 3.4E+04 Sr-90(3) Sr-90(3) 4.1 4.1E+00 E+OO 3.7E+00 3.7E+00 4.7E+03 4.7E+03 4.7E+02 4.7E+02 Tc-99 Tc-99 2.1E+01 2.1E+01 1.9E+01 1.9E+01 6.6E+05 6.6E+04 6.6E+04 U-232 U-232 1.5E+00 1.5E+00 1.4E+00 1.4E+00 2.2E+02 2.2E+01 U-233 U-233 8.3E+00 7.5E+00 7.5E+00 2.2E+04 2.2E+03 2.2E+03 U-234 U-234 U-235 8.4E+00 7.6E+00 2.2E+04 2.2E+04 2.2E+03 2.2E+03 3.5E+00 3.1E+00 3.1E+OO 2.3E+03 2.3E+02 2.3E+02 U-238 9.8E+00 8.9E+00 8.2E+03 8.2E+02 8.2E+02 • lla, NOTES: (1) The NOTES : (1) The base-case base-case values values are the lowest lowest values from from Table Table 5-1 5-11a. th e combined combined base base case in this this table table (the lowest DCGLs in in the various various (2) The Th e results results for the analysis of the streams. analyses analyses for subsurface subsurface soil) and and the th e recreationist recreationist in in the area of the streams. (3) These These DCGLs DCGLs apply apply in in the year year 2041 204 1 and and later. later. (3) 5.4 Cleanup Cleanup Goals and Additional Additional Analyses Analyses remediation of surface This section (1) (1) identifies the cleanup goals to be used used in remediation surface soil, soil , goals; (2) subsurface subsurface soil, soil , and streambed streambed sediment sediment and and the basis basis for these cleanup goals; (2) describes describes how the DCGLs and the cleanup cleanup goals will be later later refined; refined ; (3) (3) discusses use use of surrogate radionuclides;; and (4) identifies surrogate radionuclides identifies plans for the dose dose assessment of the the remediated remediated WMA 1 and WMA 22 areas. areas. 5.4.1 Cleanup Goals Goals As explained explained in in Section Section 5.1.6, 5.1.6, the dose dose modeling modeling process includes includes establishing cleanup cleanup goals below the DCGLs developed developed to meet the 25 mrem per year unrestricted unrestricted dose limit limit that are to be used used to guide remediation remediation efforts, efforts, considering the results of the analysis of the combined source source area exposure exposure scenario scenario described described in Section 5.3 5.3 and the ALARA ALARA Section 6. analysis described described in Section • Analysis Combined Combined Source Area Analysis 5.3, analysis of the limiting scenario for dose integration As indicated in Section 5.3, integration - aa remediated resident farmer living on the remed iated project premises premises who spends time in the vicinity of hiking, fish fishing, ing , and hunting - produced lower DCGLw DCGLw Erdman Brook and Franks Creek hiking, in the area of the for the recreationist groups, with the reduction values for both critical groups, reduction the percentage. streams being a much greater greater percentage. Analysis ALARA Analysis soil,, Section Section 6 describes the process used to evaluate whether whether remediation of surface soil subsurface soil, and streambed sediment below DCGLs based on 25 mrem/y would be be subsurface analyses. Section 6 standard NRC methodology for ALARA analyses. cost-effective, following the standard cost-effective, Revision 2 5-60 5-60 • WVDP PHASE 11 DECOMMISSIONING DECOMMISSIONING PLAN • be provides the results of a preliminary preliminary analysis analysis and provides provides for a final ALARA analysis to be decommissioning work. work. performed during during the Phase 1 decommissioning The preliminary ALARA ALARA analysis suggests suggests that the costs of removing slightly contaminated soil or sediment at concentrations concentrations below the DCGLs DCGLs for 25 mrem mrem per year will outweigh the benefits. That is, subsurface soil, and stream is, areas where surface surface soil, subsurface remediated to radioactivity concentrations sediment are remediated concentrations at the DCGLs satisfy the ALARA ALARA criteria.. The evaluation criteria evaluation process balances the cost of offsite disposal of additional radioactively contaminated contaminated soil (cost of $6.76 per cubic foot) and the benefits of reduced person-rem as set forth in NRC guidance). dose (benefit of $2000 per person-rem The final ALARA decommissioning ALARA analysis that will be performed performed during the Phase 1 decommissioning activities will make use of updated information information,, such as actual rather than predicted waste disposal costs. costs. However, the results will likely be similar to the preliminary preliminary analysis. Section 6 explains that the methods to be used in remediation remediation of contaminated contaminated soil and sediment, which involve excavation excavation of the material in bulk quantities, will generally generally material than necessary necessary to meet the DCGLs. DCGLs. As noted in Section 6, 6, NRC remove more material recognizes that soil excavation is a coarse removal process that is likely to remove large likely large recognizes contaminated soil and sediment fractions of the remaining remaining radioactivity radioactivity (NRC 1997). The contaminated sediment removal method is therefore expected to produce residua residuall radioactivity concentrations concentrations well therefore expected below the DCGLs. DCGLs. Cleanup Goals Goals Cleanup • Demonstration that the decommissioning Demonstration decommissioning activities have achieved the desired desired dosebased criteria is through the process described Radiation Survey and described in the Multi-Agency Radiation Site Investigation Manual Site Manual (MARSSIM) (NRC 2000). This process is outlined in Section 9, which describes describes the general content of the Phase 1 Final Status Plan.. The Phase 1 Status Survey Plan Final Status Survey Plan provides provides the details. details. For surface surface soils and sediments in the WVDP Phase 1 areas, the field cleanup goal need not be too far below the DCGL, ifif at all. As discussed previously, previously, bulk excavation excavation will generally remove necessary to meet the DCGL, DCGL, so it is likely that the remove more material material than necessary the post-remediation average concentration chosen.. post-remediation average concentration will be below whatever whatever in-process in-process goal is chosen And the costs for additional additional remediation remediation of aa surface soil or sediment site, site, while extra, are not unusually high. high . However, for subsurface soils aa field cleanup cleanup goal should be well below the DCGL remediation were necessary necessary to an because of the large costs to be incurred if additional remediation Re-excavating to depth with shoring, engineering area that failed the statistical testing. testing . Re-excavating engineering controls, and management management or disposal of extensive overburden overburden would be expensive expensive controls, compared to excavating excavating some additional material in the original remediation. Consideration goals Consideration of such factors factors led to DOE establishing in this plan the cleanup goals soil cleanup goals apply only to areas of the the shown in Table 5-14. Note that the surface soil project premises premises where there is no subsurface subsurface soil contamination contamination and that the subsurface subsurface soil cleanup goals apply only to the bottoms and lower sides (extending from aa depth of three feet and greater) of the large excavations excavations in WMA 1 and WMA 2. 2. • Revision 2 5-61 DECOMMISSIONING PLAN WVDP PHASE 1 DECOMMISSIONING 1 Remediation in in pCi/g0 pCi/g(1 )) Table 5-14. Cleanup Goals to be Used in Remediation Streambed Soil(3) Subsurface Soil(3) Surface Soil(2) SOil(2) Subsurface Streambed Sediment(2) Sediment(2) Surface Nuclide CG.w CG CGEMC CG EMC CGM CG w Am-241 Am-241 2.6E+01 3.9E+03 2.8E+03 C-14 1.SE+01 1.5E+01 1.6E+06 4.SE+02 4.5E+02 Cm-243 3.1E+01 3.1E+01 7.SE+02 7.5E+02 S.OE+02 5.0E+02 Cm-244 5.8E+01 S.8E+01 1.2E+04 9.9E+03 Cs-137(4) 1.4E+01 3.OE+02 3.0E+02 1.4E+02 1-129 1-129 2.9E-01 6.0E+02 6.0E+02 Np-237 Np-237 2.3E-01 2.3E-01 Pu-238 Pu-239 3.6E+01 2.3E+01 2.3E+01 Pu-240 2.4E+01 Pu-241 Pu-241 4 Sr-90(4) CGEMC CG EMC CG,w CG CGEMC CG EMC 1.2E+04 1.OE+03 1.0E+03 2.IE+04 2.1E+04 8.OE+04 1.8E+02 1.8E+02 S.9E+OS 5.9E+05 4.0E+03 4.OE+03 3.1E+02 3.1E+02 2.8E+03 4.5E+04 4.SE+04 3.8E+03 3.8E+03 3.6E+05 3.6E+OS 1.7E+03 1.OE+02 1.0E+02 9.4E+02 3.4E+00 3.4E+OO 3.4E+02 7.9E+01 7.9E+01 2.OE+04 2.0E+04 7.5E+01 7.SE+01 4.5E-01 4 .SE-01 4.3E+01 3.2E+01 1.1E+03 1.1E+03 7.6E+03 S.9E+03 5.9E+03 2.8E+04 1.2E+03 6.9E+03 1.4E+03 2.6E+04 1.2E+03 1.7E+05 1.7E+OS 1.7E+05 1.7E+OS 6.9E+03 1.5E+03 1.SE+03 2.6E+04 1.2E+03 1.7E+05 1.7E+05 1.OE+03 1.0E+03 1.3E+05 1.1E+05 E+OS 1.1 6.8E+05 3.4E+04 7.5E+05 Sr-90( ) 3.7E+00 3.7E+OO 7.9E+03 1.3E+02 1.3E+02 7.3E+03 4.7E+02 7.1E+04 Tc-99 1.9E+01 2.6E+04 2.7E+02 1.5E+04 6.6E+04 4.2E+06 U-232 U-232 U-233 U-233 1.4E+00 1.4E+OO 5.9E+01 3.3E+01 4.2E+02 2.2E+01 7.5E+00 7.5E+OO 8.OE+03 8.6E+01 9.4E+03 2.2E+03 2.1E+02 2.1E+02 4.4E+04 U-234 7.6E+00 7.6E+OO 1.6E+04 1.6E+04 9.0E+01 9.4E+03 2.2E+03 2.1E+05 2.1E+OS U-235 3.1E+00 3.1E+OO 6.1E+02 9.5E+01 9.SE+01 3.3E+03 2.3E+02 2.OE+03 2.0E+03 U-238 U-238 8.9E+00 8.9E+OO 2.9E+03 9.5E+01 9.SE+01 9.9E+03 8.2E+02 8.2E+03 NOTE: NOTE: (1) These cleanup goals (CGs) are are to be used as as the criteria for for the remediation activities descnbed described in in sediment cleanup cleanup goals will support Section 7 of this th is plan. plan. Note Note that the streambed sediment support unrestricted unrestricted release of the project project premises but will not necessarily necessarily support restricted release alternatives alternatives due to continued 5.2.2. the con tinued presence of Phase 2 sources as discussed in Section 5.2.2. surface soil and streambed sediment dose values for surface sediment are are the same same as the limited dose (2) The CGw CG w values assessment 5-13, values assessment DCGL values in the third and fifth columns columns of Table Table 5· 13. respectively. respectively . The CGEMC CG EMC values are based on the limiting case among the probabilistic analysis resident farmer analysis, the farmer analysis. analysis, and the deterministic residential residential gardener analysis. analysis. deterministic resident resident farmer analysis. factor reduced by aa fa ctor (3) These CGw CGw values are the assessment values in the third column of Table 5-12 reduced of 0.50 as discussed below. The DCGL DCGLEMc discussed below. EMc values are the limiting values from the multi-source farmer/residential gardener analysis or the deterministic deterministic resident farmerlresidential gardener deterministic analyses using the 1 m22 area factor from Table 9-2. the 9-2. The subsurface subsurface soil cleanup cleanup goals apply only to the bottoms of the m WMA 1 and WMA 22 deep excavations excavations and to the sides of these excavations more than three feet surface. below the ground ground surface. is, they incorporate incorporate a (4) The cleanup goals for Sr-90 and Cs-137 apply to the year 2041 204 1 and later, later. that is. 30-year decay 2011.. The 30-year selected for these key radionuclides radionuclides 30-yea r decay period was selected decay period from 2011 because of their short half-life. half-life. As noted previously, previously. the Phase Phase 2 decision decision could be made within 10 decision. years of issue of the Record of Decision and Findings Statement Statement documenting documenting the Phase 1 decision. If this approach were to involve unrestricted unrestricted release site, achieving this condition be release of the site. condition would be If expected to take more than 20 years due to the large scope of effort to exhume the underground waste It is therefore therefore highly unlikely that conditions for unrestricted unrestricted release of the the waste tanks and the NDA. It project premises could be established established before 2041, 2041 . If If Phase 2 were to involve closing radioactive radioactive place, then institutional 2041.. DOE will be responsible responsible facilities in place. institutional controls would remain in place after 2041 maintaining monitoring and for mainta ining institutional control of the project premises and providing for monitoring maintenance of the project project premises premises until completion of Phase 22 of the decommissioning. decommissioning . maintenance • 0 0 • The basis for these cleanup cleanup goals is as follows. Compliance Compliance with the cleanup cleanup goals present will be determined determined by use radionuclides are present used for remediation remediation when mixtures of radionuclides of the sum-of-fractions approach approach.. Revision 2 Revision 5-62 5-62 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • Basis for Cleanup Goals for Surface Surface Soil The surface CGw DCGL w Assessment Assessment surface soil CG values in the Surface Soil DCGLw w values are the values 5-13 . DOE considers these goals to be conservative conservative and appropriate appropriate to column of Table 5-13. remediation of surface surface soil and sediment in drainage ditches on on provide assurance assurance that any remediation the project premises premises that may be accomplished during Phase 1 of the decommissioning decommissioning will 20.1402, should the the support releasing the remediated areas areas under under the criteria of 10 CFR 20.1402, eventually determine that appropriate licensee eventually determine approach to be appropriate the for Phase 2 of the 17 decommissioning..17 decommissioning Basis for Cleanup Goals for Subsurface Soil DOE has established the subsurface soil cleanup goals at 50 percent percent of subsurface soil DCGLs calculated in the limited site-wide dose assessments for 22.5 22.5 mrem per year (Table (Table 5-12). 5-12). The cleanup goals for subsurface subsurface soil will therefore equate to 11.25 mrem per year. approach to provide DOE is taking this approach provide additional additional assurance assurance that remediation remediation of the WMA 1 and WMA 2 excavated excavated areas will support all potential options for Phase 2 of the the decommissioning. As indicated previously, these cleanup goals apply only to the bottom bottom of decommissioning . previously, the large WMA 1 and WMA 2 excavations and to the sides of these excavations excavations three feet or more below the surface. surface. Streambed Sediment Basis for Cleanup Goals for Streambed Sediment DCGLw site-wide dose assessment (the last DOE has used the DCGL w values from the limited site-wide column in Table 5-12 and Table 5-13) as the cleanup goals for streambed sediment. These These cleanup values are substantially less than those developed developed for the base-case recreationist scenario base-case recreationist and are considered considered to be supportive of any approach that may be selected for Phase 2 of decommissioning. the decommissioning. • As noted in the discussion on the ALARA analysis results, DOE expects that the actual levels of residual remediation,, residual radioactivity radioactivity will turn out to be less than the DCGLs used for remediation i.e., be i.e., these cleanup cleanup goals, goals, owing to the characteristics characteristics of the remediation method to be used. 5.4.2 Refining DCGLs and Cleanup Cleanup Goals Goals The calculated DCGLs for 25 mrem per year and the associated cleanup goals will be be refined as appropriate after the data from the soil and sediment characterization program refined sediment characterization program to be completed early in Phase 1 of the decommissioning becomes becomes available. These data are expected to provide additional additional insight into the radionuclides radionuclides of interest in environmental media and the depth and areal distribution of the contamination. contamination . Such information could, could , for example, lead to deleting one or more radionuclides from further consideration in the Phase example, deleting more radionuclides consideration 1 cleanup or lead to more realistic source geometry for development development of DCGLs for surface surface soil contamination.. Analytical data from the subsurface characterization measurements measurements soil contamination subsurface soil soil characterization being taken in 2008 2008 could also provide information to help help refine the subsurface soil DCGLs. DCGLs. As noted previously, surface soil may or may not be remediated in Phase 1 of the decommissioning. As noted previously, surface soil mayor may not be remediated in Phase 1 of the decommissioning. However, characterization performed early in However, it it is is possible possible that that characterization in Phase 1 could identify surface soil contamination that that would warrant warrant remediation to to reduce radiation doses during the period between Phase 1 contamination and Phase 2 of the decommissioning. decommissioning. In In the unlikely developed, the areas of unlikely event event that this situation developed, concern remediated in in Phase 1. concern would be remediated 17 17 • Revision 2 5-63 5-63 WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN If leads to refinement of the DCGLs and cleanup cleanup goals, then If evaluation of the new data leads accordingly to reflect the new values. this plan will be revised accordingly values. Since such a change could affect the project end conditions, conditions, the plan revision would be provided provided to NRC for review and input prior to issue following the change change process described in Section 1. 5.4.3 Use of a Surrogate Surrogate Radionuclide DCGL • A surrogate radionuclide is aa radionuclide surrogate radionuclide radionuclide in a mixture of radionuclides whose concentration measured and can be used to infer concentration is easily measured infer the concentrations concentrations of the other radionuclides If actual radioactive radionuclides in the mixture. mixture. If radioactive contamination contamination levels levels of the surrogate surrogate radionuclide are below the specified concentration, then the sum radionuclide below concentration , of doses from all 18 radionuclides limit.18 radionuclides in the mixture will fall below the dose limit. The tables in this section do not provide DCGLw surrogate radionuclide radionuclide DCGL w values for aa surrogate because radionuclide distributions distributions in soil and sediment are not sufficient because available data on radionuclide However, surrogate radionuclide DCGLw cleanup goals will to support this. this. However, radionuclide DCGL w values for the cleanup be developed incorporated into this section ifif evaluation additional characterization developed and incorporated evaluation of additional data shows that Cs-137 or another easy easy to measure measure radionuclide radionuclide can be used effectively as as a surrogate for all radionuclides in source radionuclides in source soil, soil , subsurface subsurface soil, soil , and/or and/or streambed sediment streambed sediment in an area. area. 5.4.4 Preliminary Assessment Preliminary Dose Assessment Preliminary dose assessments assessments have been performed performed for the remediated WMA WMA 1 and WMA 2 excavations. These assessments made use of the maximum maximum measured radioactivity concentration in the Lavery till for each radionuclide radionuclide as summarized in Table 51, and the results of modeling modeling to develop DCGLs for 25 mrem per year and the multisource analysis results as shown in Table 5-1 5-11lc. c. The results were as follow: WMA 1, a maximum maximum of approximately approximately 88 mrem a year WMA 2, 2, a maximum approximately 0.2 maximum of approximately 0.2 mrem a year Given Given the limited data available, available, these results must be viewed as order-of-magnitude order-of-magnitude estimates. However, they do suggest that actual potential doses from the two remediated remediated areas areas are likely to be substantially substantially below 25 mrem per year. Note that the primary primary dose dose driver approximately 66 percent of the the driver for these estimates estimates is Sr-90, Sr-90, which accounts for approximately estimated dose for the WMA 1 excavation and approximately approximately 61 percent of the estimate for the WMA 2 excavation. excavation . • NOTE NOTE The use of maximum rather than average values in these dose estimates adds adds conservatism, including values that are simply detectable conservatism, as does including simply the highest minimum detectable concentrations, especially in the case of Np-237. Np-237. (There was a wide range of several orders of magnitude among the minimum detectable detectable concentrations concentrations reported reported for the the 2008 sample data.) data.) As with the DCGLs, DCGLs, decay of Sr-90 and Cs-137 over 30 years is accounted accounted for in the estimate. 18 Guidance on the use of surrogate measurements provided in Section 4.3.2 of NUREG-1575, Multi-Agency Guidance on the use of surrogate measurements provided in Section 4 .3.2 of NUREG-1575, Multi-Agency Radiation Survey Survey and Site Investigation Investigation Manual (NRC 2000) would would be be followed followed.. Radiation Manual (MARSSIM) (MARSSIM) (NRC 18 Revision 2 5-64 • WVDP PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN • As noted previously, previously, DOE will perform residual radioactivity perform aa dose assessment assessment for the residual excavated areas using Phase 1 final status survey data data.. This in the WMA 1 and WMA 2 excavated This assessment will use the same methodology used in in development subsurface soil development of the subsurface DCGLs to estimate estimate the potential radiation dose using the actual measured residual radioactivity concentrations. The results of the dose assessment radioactivity assessment will be made available to stakeholders. Note that a more-comprehensive more-comprehensive dose assessment NRC and other stakeholders. assessment that also performed in connection with Phase 2 of takes into account account the Phase 22 sources may be performed phase. depending on the approach selected for that phase. the decommissioning, decommissioning, depending 5.5 Monitoring, Controls Monitoring, Maintenance, Maintenance, and Institutional Controls Inherent in the use of the 30-year 30-year decay period used used in development development of DCGLs and cleanup goals for Sr-90 and Cs-137 Cs-137 is the assumption that all or part of the project unrestricted use before 2041. 2041 . DOE will be responsible for premises will not be released for unrestricted maintenance of the project premises and for maintaining institutional monitoring and maintenance controls until completion completion of Phase 2 of the WVDP decommissioning, decommissioning, which is assumed to to If aa occur after 2041 if unrestricted release criteria. if Phase Phase 2 were to be designed to meet unrestricted criteria . If 2, then institutional controls are assumed close-in-place close-in-place approach approach was selected for Phase 2, to be required beyond 2041. 2041 . 5.6 References References Code of Federal Federal Regulations Regulations CriteriaFor Termination (LTR). 10 CFR 20, Subpart E, Radiological Radiological Criteria For License Termination (L TR) . • 10 CFR 20.1003, 20 .1003, Definitions. Definitions. DOE Orders Orders U.S, ProtectionProgram, DOE Order 450.1, 450.1, Environmental Environmental Protection Program, including including Changes 1 and 2. U.S, Energy, Washington, 2003.. January 15, 2003 Department of Energy, Washington, D.C. January and the Environment, Radiation Protection DOE Order 5400.5, Radiation Protection of the Public Public and Environment, Change Change 2. U.S,, Department Washington, D.C., January 7, 1993. 1993. U.S Department of Energy, Energy, Washington, DOE Technical Technical Standards Standards 1153-2002, A Graded GradedApproach for Evaluating Evaluating Radiation Doses to Aquatic DOE Standard Standard 1153-2002, Radiation Doses and Terrestrial TerrestrialBiota. U.S, Department Department of Energy, Washington, and Biota. U.S, Washington , D.C., July July 2002. 2002 . Other Other References References ParameterAnalysis, Analysis, Radioactivity from Decommissioning, Decommissioning, Parameter Beyeler, et al. 1999, Residual Residual Radioactivity A. NUREG/CR-5512, Vol 3, Draft Report for Comment. Beyeler, W. W. E., W. W. A. NUREG/CR-5512, T. J. Brown, E. Kalinina, D. P. Gallegos, Hareland, F. F. A. A. Duran, Duran , T. J. Brown, Gallegos, and P. A. Davis, Mexico, October Sandia Sandia National Laboratories, Albuquerque, Albuquerque, New Mexico, October 1999. Dames and Moore 1994, North North Plateau Plateau Groundwater Groundwater Seepage Survey, Letter Report D&M:SPV:PJG:1 1B:0249. Dames and Moore, West Valley New York, D&M :SPV:PJG :11B:0249. York , August 15, 15, 1994. • Revision 2 5-65 5-65 WVDP WVDP PHASE PHASE 1 DECOMMISSIONING DECOMMISSIONING PLAN PLAN DOE DOE 2004, 2004, Users Guide, RESRAD-BIOTA: RESRAD-BIOTA : A A Tool for Implementing a Graded Graded Approach Approach to to Biota Dose Evaluation, Evaluation , Version Version 1, 1, DOE/EH0676. DOE/EH0676. Environmental Environmental Assessment Assessment Division, Division, Argonne Argonne National National Laboratory, Laboratory, Argonne, Argonne , Illinois, Illinois, January January 2004. 2004. EPA 1997, 1997, Exposure Exposure Factors Factors Handbook. National National Center for for Environmental Environmental Assessment, Assessment, S. Environmental Environmental Protection Protection Agency, Agency, Office of of Research Research and and Development, Development, U. S. Office Washington , D.C., D.C. , 1997. 1997. Washington, • Hemann of the Core Area Area of the North Hemann and and Steiner Steiner 1999, 1999, 1998 Geoprobe Geoprobe Investigation Investigation of Plateau Plateau Groundwater Groundwater Plume, Plume , WVDP-346, WVDP-346, Revision Revision 0. O. Hemann, Hemann , M.R. and and R.E. R.E. Steiner II, II , West West Valley Nuclear Nuclear Services Company, Company, June June 11, 11 , 1999. 1999. Dispersion of Effluents NRC NRC 1977, Estimating Estimating Aquatic Aquatic Dispersion Effluents from Accidental and Routine Reactor Regulatory Guide Releases for the Purpose Appendix I, I, Regulatory Guide 1.113, 1.113, Purpose of Implementing Appendix Rev. 1. U.S. U.S. Nuclear Nuclear Regulatory Rev. 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Price, Plant Process Building, Calculation Plant Process Calculation DPlan-SAIC-JDP-003. Price , J., 2009. Maryland, October Corporation, Germantown, Applications International Appl ications Corporation , Germantown , Maryland, 2009. 8.10),, University Manual for SIBERIA (Version 8.10) 2000, User User Manual Willgoose 2000, SIBERIA (Version University of Newcastle, New Australia, July 2000. South Wales, Wales, Environmental Demonstration Project WVES and URS 2009, 2009, West Valley Demonstration Project Annual Site Environmental and URS URS Valley Environmental Services Calendar Year 2008. West Report, Calendar Report, Environmental Inc.,, West Valley, Valley, New York, Group, Inc. York, September 2009. Part 4 Ill Hydrology Information Document Document Volume III 1993a. Environmental Environmental Information WVNSCO 1993a. Hydrology Part 0. West and Geochemistry, Geochemistry, WVDP-EIS-009, Revision O. Groundwater Hydrology Hydrology and Groundwater 19, 1993. 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Sciences Division, Argonne National • • Yu, et al. 2000, Development Development of Probabilistic Probabilistic RESRAD and RESRAD-BUILD 3.0 RESRAD 6.0 and Computer Codes, NUREG/CR-6697, NUREG/CR-6697, ANL/EAD/TM-98. Computer Codes, ANUEADITM-98. Yu, Yu, C., et al., aI., Environmental Environmental Assessment Division, Argonne National Laboratory, Argonne, Illinois, Illinois, November 2000. Yu, et al. 2001, 2001, User's User's Manual ANUEAD-4. Yu, C., et al., aI., Manual for RESRAD RESRAD Version 6, ANL/EAD-4. Environmental Environmental Assessment Division, Argonne National Laboratory, Argonne, Illinois, July 2001. 2001. Revision 2 5-67 5-67 This page is intentionally intentionally blank. • • •