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Validation of the efficiency of a decontamination process
23/11/2010
-1-
Validation of the efficiency of a decontamination process
using ozone for EURO MVP
Study performed
By
2010 September to November
Laboratoire SILLIKER
Laboratoire de Microbiologie - Unité R&D
10, rue les Châteaux Saint Sylvère
95011 CERGY Cedex
FRANCE
Technical contact
Aurélie PERNOT
Research engineer
Phone : 33 (0)1 30 75 61 56
E-mail : [email protected]
Joël CROCIANI
Expert on microbiology Project
Phone : 33 (0) 1 34 41 13 36
E-mail : [email protected]
Customer
Euro MVP
2, Chemin des Cossins
60750 Choisy au Bac
FRANCE
http://www.euromvp.com
Mr Olivier VANCOILLIE
Phone : 06 38 84 53 58
[email protected]



23/11/2010
-2-
CONTENTS
I.
SUMMARY................................................................................................................................................... 3
II.
MATERIAL AND METHODS............................................................................................................... 3
II.1.
MEASURE OF THE BACTERIAL DESTRUCTION ON A SURFACE .................................................................. 3
II.1.1.
Surface .......................................................................................................................................... 3
II.1.2.
Ozone system................................................................................................................................. 3
II.1.3.
Choice of strains ........................................................................................................................... 3
II.1.4.
Analysis method ............................................................................................................................ 4
II.1.5.
Protocol ........................................................................................................................................ 4
II.1.6.
Calculation of the percentage of bacterial reduction ................................................................... 5
II.2.
MEASURE OF BACTERIAL REMOVAL OF LEGIONELLA PNEUMOPHILA...................................................... 6
II.3.
STUDY OF THE EFFECT OF THE TREATMENT ON A BIOFILM ...................................................................... 6
II.3.1.
III.
Choice of the strain....................................................................................................................... 6
RESULTS ................................................................................................................................................. 7
III.1.
MEASURE OF THE BACTERIAL DESTRUCTION ON A SURFACE .................................................................. 7
III.1.1.
Escherichia coli ............................................................................................................................ 7
III.1.2.
Listeria monocytogenes ................................................................................................................ 7
III.1.3.
Bacillus cereus.............................................................................................................................. 8
III.1.4.
Staphylococcus aureus.................................................................................................................. 9
III.1.5.
Yeast.............................................................................................................................................. 9
III.1.6.
Mould.......................................................................................................................................... 10
III.2.
INTERPRETATION OF RESULTS .............................................................................................................. 10
III.3.
MEASURE OF THE BACTERIAL REDUCTION OF LEGIONELLA PNEUMOPHILA ...................................... 11
III.4.
STUDY OF THE EFFECT OF THE TREATMENT ON A BIOFILM .................................................................... 12



23/11/2010
I.
-3-
SUMMARY
This report presents the protocol details and the results of validation study performed by
SILLIKER for Euro MVP. This study consists in validating a decontamination process using
ozone. The process is estimated for different germs on a plastic surface. The study consists
in contaminating artificially the surface with a germ. The contamination allows to calculate the
microbial reduction for each germs.
II. MATERIAL AND METHODS
II.1. MEASURE OF THE BACTERIAL DESTRUCTION ON A
SURFACE
II.1.1.
SURFACE
A plane surface in plastic of 1000 cm² (25 x 40 cm) is used.
II.1.2.
OZONE SYSTEM
The ozone system model WMS (Brand GO3) is used.

II.1.3.
CHOICE OF STRAINS
The selected germs are bacteria linked to food-borne illness and/or responsible of spoilage.
Yeasts and moulds represent a spoilage flora for fruit and vegetables so they will be studied
too.
The selected germs are:
 Escherichia coli
 Listeria monocytogenes
 Bacillus cereus
 Staphylococcus aureus
 Yeast : Saccharomyces cerevisiae
 Mould : Aspergillus niger



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II.1.4.
ANALYSIS METHOD
Analyses are performed according to methods in the table below:
Parameters
Methods
Escherichia coli
NF ISO 16649-2
Listeria monocytogenes
RAPID'L mono (BRD-07/05-09/01)
Bacillus cereus (spore)
ISO 7932
Bacillus cereus (cell)
ISO 7932
Staphylococcus aureus
NF V 08-057-1
Yeast
NF V08-059
Mould
NF V08-059
II.1.5.
PROTOCOL
The surface is artificially contaminated by microbial suspension obtained by transplanting a
colony on a tube of culture media. The required inoculation level is between 105 and 107
CFU/1000cm². The inoculation is performed in order to contaminate the surface
homogeneously. A plastic surface of 1000 cm² is used. The suspension is spread on the
surface and allowed to dry 30 minutes in a sterile atmosphere thanks to Bunsen burner. After
inoculation, germs remaining on the surface are removed with a sterile wipe which is plunge
into diluent. The suspension is spread on plates for enumeration. This enumeration indicates
the contamination level before treatment (called Control). For each germ, 3 controls are
performed.
a. Treatment with Ozoned water
The inoculated surface is treated with ozone: ozoned water is applied perpendicularly at
about 20 cm of the surface during 30 seconds, then the inoculated germ remaining on the
surface is enumerated: this enumeration indicates the level of residual contamination. For
each germ, 3 repetitions of the test are performed.
In order to check if the bacterial removal is due to ozone or if it is due to the pressure of the
ozoned water, a test is carried out using tap water with E. coli, L. monocytogenes, S. aureus
and S. cerevisiae. The final pipe of the equipment is connected to the faucet (so the water is
not ozoned). As the water goes through the same pipe (same length, same diameter) the
flow of tap water is the same that the flow of ozoned water. The tap water is applied during
30 seconds on the inoculated surface.



23/11/2010
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b. Treatment with a disinfectant
3 repetitions of the test are carried out treating the surface with a disinfectant: Amphospray
41 (disinfectant to be spray) of Laboratoires ANIOS, in order to compared the efficacy of the
process to a disinfectant.
In the same way, the suspension is spread on the surface and allowed to dry 30 minutes in a
sterile atmosphere thanks to Bunsen burner. The disinfectant (4 mL) is sprayed uniformly on
the surface and allowed to dry 5 minutes. Germs remaining on the surface are enumerated.
For each germ, 3 repetitions are performed.
Amphospray 41:
Composition: Denatured ethanol (41 % v/v), polyhexamethylene biguanide hydrochloride, N(3-aminopropyl)-N-dodecylpropane-1,3-diamine,
didecyldimethylammonium
chloride,
excipients.
Instructions for use: Ready-to-use solution for professional use. Spray uniformly to obtain an
even antimicrobial film. Allow to dry, do not rinse. Used 30 à 40 mL/m²
Microbiological properties: Bactericidal: EN 1040, T 72-301, NF T 72-171, NF T 72-190.
Active against MRSA (EN 13727) and Mycobacter tuberculosis (B.K).
Fungicidal activity (C. albicans): EN 1275.
Active against HIV-1, HBV and Rotavirus.
II.1.6.
CALCULATION OF THE PERCENTAGE OF BACTERIAL
REDUCTION
Percentage of bacterial reduction = ((Median of Controls – residual concentration) / Median
of Controls) x100



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II.2. MEASURE OF BACTERIAL REMOVAL OF LEGIONELLA
PNEUMOPHILA
The study is performed with Legionella pneumophila.
The microbial suspension is obtained by transplanting a colony on a tube of culture media.
The suspension is ½ diluted with ozoned water and allow in contact during 1 hour. The
Control is perfomed with tap water instead of ozoned water. Three enumerations are
performed after 1 minute, 30 minutes and 1 hour of contact.
The concentration of Legionella pneumophila before and after treatment is indicated. These
results allow to calculate logarithmic reduction due to the decontamination treatment.
Parameter
Method
Legionella pneumophila
NF T90-431
II.3. STUDY OF THE EFFECT OF THE TREATMENT ON A
BIOFILM
II.3.1.
CHOICE OF THE STRAIN
The study concerns the strain which resists the most at the ozone treatment, here spores of
Bacillus cereus.
The surface is artificially contaminated overnight with spores of Bacillus cereus. The required
inoculation level is between 105 and 107 CFU/1000cm². A plastic surface of 1000 cm² is
used. The surface is washed with ozoned water during 30 seconds. Germs remaining on the
surface are removed with a sterile wipe which is plunge into diluent. The suspension is
spread on plates for enumeration. This enumeration indicates the contamination level after
treatment. The control (before treatment) is performed in the same way but without the
ozoned water.
The concentration of the germ before and after treatment allows to calculate logarithmic
reduction due to the decontamination treatment.



23/11/2010
-7-
III. RESULTS
III.1. MEASURE OF THE BACTERIAL DESTRUCTION ON A
SURFACE
III.1.1. ESCHERICHIA COLI
Result Residual flora
cfu/1000cm²
Log cfu/1000cm²
Control 1
140 000 000
8.15
144 000 000
8.16
Control 2
Control 3
148 000 000
8.17
Tap water
2900
3.46
1400
3.15
2200
3.34
Ozoned water
2600
3.41
190
2.28
Disinfectant
260
2.41
Amphospray 41
300
2.48
The Median of the 3 repetitions is in bold.
Protocol
% of bacterial
reduction
99.99
99.99
99.99
99.99
99.99
99.99
99.99
Median of Controls = 144 000 000 cfu/1000 cm²
Average of bacterial reduction: 99.99% for Ozoned water and Disinfectant.
The residual flora after using the disinfectant is 1 Log cfu/1000cm² lower than the residual
flora after treatment with ozoned water. There is no difference between the results of residual
flora for tap water and ozoned water.
III.1.2. LISTERIA MONOCYTOGENES
Result Residual flora
cfu/1000cm²
Log cfu/1000cm²
120 000 000
8.08
Control 1
Control 2
123 000 000
8.09
Control 3
102 000 000
8.01
Tap water
3700
3.57
200
2.30
Ozoned water
~40
1.60
710
2.85
28 000
4.45
Disinfectant
~20
1.30
Amphospray 41
~30
1.48
The Median of the 3 repetitions is in bold
Protocol
% of bacterial
reduction
99.99
99.99
99.99
99.99
99.98
99.99
99.99
Median of Controls = 120 000 000 cfu/1000 cm²
Average of bacterial reduction: 99.99% for Ozoned water and Disinfectant.
The residual flora after treatment with ozoned water is 1 Log cfu/1000cm² lower than residual
flora after treatment with tap water. There is no difference between the results of residual
flora for disinfectant and ozoned water.



23/11/2010
-8-
III.1.3. BACILLUS CEREUS
Cells of Bacillus cereus:
Result Residual flora
cfu/1000cm²
Log cfu/1000cm²
Control 1
~13 000
4.11
Control 2
~15 000
4.18
~14 000
4.15
Control 3
~70
1.85
~30
1.48
Ozoned water
~30
1.48
<10
1
Disinfectant
<10
1
Amphospray 41
<10
1
The Median of the 3 repetitions is in bold
Protocol
% of bacterial
reduction
99.50
99.79
99.79
99.93
99.93
99.93
Median of Controls = 14 000 cfu/1000 cm²
Average of bacterial reduction: 99.69% for Ozoned water and 99.93% for Disinfectant.
The residual flora after using disinfectant is lower than residual flora after treatment with
ozoned water.
Spores of Bacillus cereus:
Result Residual spore
cfu/1000cm²
Log cfu/1000cm²
Control 1
18 000
4.26
~12 000
4.08
Control 2
Control 3
~7000
3.85
220
2.34
Ozoned water
210
2.32
310
2.49
510
2.71
Disinfectant
94
1.97
Amphospray 41
790
2.90
The Median of the 3 repetitions is in bold
Protocol
% of bacterial
reduction
98.17
98.25
97.42
95.75
99.22
93.42
Median of Controls = 12 000 cfu/1000 cm²
Average of bacterial reduction: 97.95% for Ozoned water and 96.13% for Disinfectant.
There is no difference between the results of residual spore obtained with the disinfectant
and the ozoned water (reduction about 2 Log cfu/1000cm² in comparison to the control).



23/11/2010
-9-
III.1.4. STAPHYLOCOCCUS AUREUS
Result Residual flora
cfu/1000cm²
Log cfu/1000cm²
Control 1
580 000
5.76
650 000
5.81
Control 2
Control 3
710 000
5.85
Tap water
2700
3.43
290
2.46
Ozoned water
220
2.34
350
2.54
~60
1.78
Disinfectant
~80
1.90
Amphospray 41
~60
1.78
The Median of the 3 repetitions is in bold
Protocol
% of bacterial
reduction
99.59
99.96
99.97
99.95
99.99
99.99
99.99
Median of Controls = 650 000 cfu/1000 cm²
Average of bacterial reduction: 99.96% for Ozoned water and 99.99% for Disinfectant.
The residual flora after using the disinfectant is 1 Log cfu/1000cm² lower than residual flora
after treatment with ozoned water.
The residual flora after treatment with ozoned water is 1 Log cfu/1000cm² lower than residual
flora after treatment with tap water.
III.1.5. YEAST
Result Residual flora
cfu/1000cm²
Log cfu/1000cm²
~5000
Control 1
3.70
~2000
Control 2
3.30
~4000
3.60
Control 3
80
Tap water
1.90
<10
1
Ozoned water
<10
1
<10
1
~150
2.18
Disinfectant
<10
1
Amphospray 41
<10
1
The Median of the 3 repetitions is in bold
Protocol
% of bacterial
reduction
98.00
99.75
99.75
99.75
96.25
99.75
99.75
Median of Controls = 4000 cfu/1000 cm²
Average of bacterial reduction: 99.75% for Ozoned water and 98.58% for Disinfectant.
The residual flora after treatment with ozoned water is lower than residual flora after
treatment with tap water.



23/11/2010
- 10 -
III.1.6. MOULD
Result Residual flora
cfu/1000cm²
Log cfu/1000cm²
34 000
Control 1
4.53
28 000
Control 2
4.45
29 000
4.46
Control 3
210
2.32
Ozoned water
350
2.54
250
2.40
~90
1.95
Disinfectant
180
2.26
Amphospray 41
~110
2.04
The Median of the 3 repetitions is in bold
Protocol
% of bacterial
reduction
99.28
98.79
99.14
99.69
99.38
99.62
Median of Controls = 29 000 cfu/1000 cm²
Average of bacterial reduction: 99.07% for Ozoned water and 99.56% for Disinfectant
There is no difference between the results of residual flora obtained with the disinfectant and
with ozoned water.
III.2. INTERPRETATION OF RESULTS
The treatment of the surface with ozoned water during 30 seconds allows a bacterial
reduction of 99.99% for Escherichia coli and Listeria monocytogenes. The same bacterial
reduction is obtained with the disinfectant Amphospray 41. However, the results obtained
with ozoned water should be discussed because the tests with tap water during 30 secondes
show also a bacterial reduction of 99.99%. So germs are removed of the plastic surface with
the pressure of the water and suspended in the air.
A treatment of the surface with ozoned water during 30 seconds allows a bacterial reduction
of 99.96% for Staphylococcus aureus, 99.75% for Saccharomyces cerevisiae and 99.07% for
Aspergillus niger.
The cells of Bacillus cereus are reduced to 99.69% and the spores of Bacillus cereus are
reduced to 97.95% thanks to the treatment with ozoned water during 30 seconds.



23/11/2010
- 11 -
III.3. MEASURE OF THE BACTERIAL REDUCTION OF
LEGIONELLA PNEUMOPHILA
Enumeration of the Legionella pneumophila suspension: 4 400 000 cfu/ml
Analysis
Enumeration of
Legionella
pneumophila in the
mix « suspension of
Legionella
pneumophila + Tap
water »
Enumeration of
Legionella
pneumophila in the
mix « suspension of
Legionella
pneumophila +
Ozoned water »
Contact
time
1 minute
30 minutes
1 hour
1 minute
30 minutes
1 hour
cfu/ml
Log
cfu/ml
2 400 000
2 600 000
2 100 000
2 500 000
2 600 000
2 300 000
2 300 000
1 900 000
2 500 000
1 900 000
2 600 000
2 700 000
2 800 000
3 200 000
1 500 000
2 300 000
1 600 000
700 000
6.38
6.41
6.32
6.40
6.41
6.36
6.36
6.28
6.40
6.28
6.41
6.43
6.45
6.51
6.18
6.36
6.20
5.85
Median after 1 hour
(Log cfu/ml)
Logreduction
(Log cfu/ml)
6.36
-
6.20
0.16
The Median of the 3 repetitions is in bold.
The mix at equal volume of Legionella pneumophila suspension and tap water has a
constant concentration during the hour of testing (Median: 2 400 000 cfu/ml). So tap water
has no effect on the concentration of Legionella pneumophila
There is no difference between the mix « suspension and ozoned water » and the mix
« suspension and tap water » for 1 and 30 minutes of contact. After one hour of contact
between the suspension and ozoned water, a decrease is detected: the log reduction is 0.16
log cfu/ml compared with the mix “suspension and tap water”. This log reduction is not
enough to ensure the total destruction of Legionella pneumophila.



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III.4. STUDY OF THE EFFECT OF THE TREATMENT ON A
BIOFILM
Result Residual flora
cfu/1000cm²
Log cfu/1000cm²
360
000
Control 1
5.56
440 000
Control 2
5.64
390 000
5.59
Control 3
27 000
4.43
37 000
4.57
Ozoned water
78 000
4.89
The Median of the 3 repetitions is in bold
Protocol
% of bacterial
reduction
93.08
90.51
80.00
Median of Controls = 390 000 cfu/1000 cm²
A treatment with ozoned water during 30 seconds allows to reduce about 1 Log cfu/1000cm²
the biofilm of Bacillus cereus spores. Without biofilm, ozoned water allows a reduction of 2
Log cfu/1000cm² of Bacillus cereus spores (Results page 8). So the effect of ozoned water is
less efficient on biofilms.



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